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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Hoye, Robert L. Z.
University of Oxford
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (26/26 displayed)
- 2024Direct linearly polarized electroluminescence from perovskite nanoplatelet superlatticescitations
- 2024Resolving electron and hole transport properties in semiconductor materials by constant light-induced magneto transportcitations
- 2024Lead‐free halide perovskite materials and optoelectronic devices: progress and prospectivecitations
- 2023Wide‐Bandgap Perovskite‐Inspired Materials: Defect‐Driven Challenges for High‐Performance Optoelectronicscitations
- 2023Wide-bandgap perovskite-inspired materials: defect-driven challenges for high-performance optoelectronicscitations
- 2023Lead‐Free Halide Perovskite Materials and Optoelectronic Devices: Progress and Prospectivecitations
- 2023The ferro-pyro-phototronic effect for high-performance self-powered photodetectorscitations
- 2022Recent Progress in Mixed A‐Site Cation Halide Perovskite Thin‐Films and Nanocrystals for Solar Cells and Light‐Emitting Diodescitations
- 2022Colloidal metal‐halide perovskite nanoplatelets: thickness‐controlled synthesis, properties, and application in light‐emitting diodescitations
- 2022Recent progress in mixed a‐site cation halide perovskite thin‐films and nanocrystals for solar cells and light‐emitting diodescitations
- 2022The effect of caesium alloying on the ultrafast structural dynamics of hybrid organic-inorganic halide perovskitescitations
- 2022Colloidal Metal‐Halide Perovskite Nanoplatelets: Thickness‐Controlled Synthesis, Properties, and Application in Light‐Emitting Diodescitations
- 2022The effect of caesium alloying on the ultrafast structural dynamics of hybrid organic–inorganic halide perovskitescitations
- 2021Defect passivation in lead‐halide Perovskite nanocrystals and thin films: toward efficient LEDs and solar cellscitations
- 2021Nickel oxide thin films grown by chemical deposition techniques: Potential and challenges in next‐generation rigid and flexible device applications
- 2021Understanding the Role of Grain Boundaries on Charge‐Carrier and Ion Transport in Cs 2 AgBiBr 6 Thin Films
- 2021High-performance self-powered photodetectors achieved through the pyro-phototronic effect in Si/SnOx/ZnO heterojunctionscitations
- 2021Understanding the Role of Grain Boundaries on Charge‐Carrier and Ion Transport in Cs<sub>2</sub>AgBiBr<sub>6</sub> Thin Filmscitations
- 2021Perovskite-inspired materials for photovoltaics and beyond—from design to devices
- 2021An interlinked computational-experimental investigation into SnS nano-flakes for field emission applicationcitations
- 2021State of the art and prospects for halide perovskite nanocrystalscitations
- 2020Bandgap lowering in mixed alloys of Cs2Ag(SbxBi1−x)Br6 double perovskite thin filmscitations
- 2018Lead-Free Perovskite Semiconductors Based on Germanium-Tin Solid Solutions:Structural and Optoelectronic Propertiescitations
- 2018Boosting Tunable Blue Luminescence of Halide Perovskite Nanoplatelets through Postsynthetic Surface Trap Repaircitations
- 2018Lead-Free Perovskite Semiconductors Based on Germanium-Tin Solid Solutionscitations
- 2013Nanostructured conformal hybrid solar cells : a promising architecture towards complete charge collection and light absorptioncitations
Places of action
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article
An interlinked computational-experimental investigation into SnS nano-flakes for field emission application
Abstract
Layered binary semiconductor materials have attracted significant interest as field emitters due to their low work function, mechanical stability, high thermal and electrical conductivity. Herein, we report a systematic experimental and theoretical investigation of SnS nanoflakes synthesized using a simple, low-cost, and non-toxic hot injection method for field emission studies. The field emission studies were carried out on SnS nanoflakes thin film prepared using a simple spin coat technique. The x-ray diffraction (XRD) and Raman spectroscopy analysis revealed an orthorhombic phase of SnS. Scanning electron microscopy (SEM) analysis revealed that as-synthesized SnS has flakes-like morphology. The formation of pure-phase SnS nanoflakes was further confirmed by x-ray photoelectron spectroscopy (XPS) analysis. The UV-Visible-NIR spectroscopy analysis shows that SnS nanoflakes have a sharp absorption edge observed in the UV region and have a band gap of ∼ 1.66 eV. In addition, the first-principles density functional theory (DFT) calculations were carried out to provide atomic-level insights into the crystal structure, band structure, and density of states (DOS) of SnS nanoflakes. The field emission properties of SnS nanoflakes were also investigated and found that SnS nanoflakes have a low turn-on field (∼ 6.2 V/μm for 10 μA/cm2), high emission current density (∼ 104 μA/cm2 at 8.0 V/μm), superior current stability (∼ 2.5 hrs for ∼ 1 μA) and a high field enhancement factor of 1735. The first principle calculations the predicted lower work function of different surfaces, especially for the most stable SnS (001) surface ( = 4.32 eV), is believed to be responsible for the observed facile electron emission characteristics. We anticipate that the SnS could be utilized for future vacuum nano/microelectronic and flat panel display applications due to the low turn-on field and flakes-like structure.