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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Verbeeck, Jo
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (22/22 displayed)
- 2024Phase coexistence induced surface roughness in V<sub>2</sub>O<sub>3</sub>/Ni magnetic heterostructurescitations
- 2024Stabilizing Perovskite Pb(Mg<sub>0.33</sub>Nb<sub>0.67</sub>)O<sub>3</sub>-PbTiO<sub>3</sub> Thin Films by Fast Deposition and Tensile Mismatched Growth Templatecitations
- 2023Low-Dose 4D-STEM Tomography for Beam-Sensitive Nanocompositescitations
- 2022On the formation mechanisms of intragranular shear bands in olivine by stress-induced amorphizationcitations
- 2021Optical versus electron diffraction imaging of Twist-angle in 2D transition metal dichalcogenide bilayerscitations
- 2021Increased performance improvement of lithium-ion batteries by dry powder coating of high-nickel NMC with nanostructured fumed ternary lithium metal oxidescitations
- 2020Single femtosecond laser pulse excitation of individual cobalt nanoparticlescitations
- 2020Reliable Characterization of Organic and Pharmaceutical Compounds with High Resolution Monochromated EEL Spectroscopycitations
- 2020Unravelling stacking order in epitaxial bilayer MX₂ using 4D-STEM with unsupervised learningcitations
- 2019Controlling the interfacial conductance in <tex>$LaAlO_{3}/SrTiO_{3}$</tex> in 90 degrees off-axis sputter depositioncitations
- 2018Getting rid of anti-solvents: gas quenching for high performance perovskite solar cellscitations
- 2017Energy level alignment and cation charge states at the <tex>$LaFeO_{3}/LaMnO_{3}$</tex> (001) heterointerfacecitations
- 2017One step toward a new generation of C-MOS compatible oxide PN junctionscitations
- 2017Direct observation of enhanced magnetism in individual size- and shape-selected 3d transition metal nanoparticlescitations
- 2016A universal deposition protocol for planar heterojunction solar cells with high efficiency based on hybrid lead halide perovskite familiescitations
- 2016Long-range domain structure and symmetry engineering by interfacial oxygen octahedral coupling at heterostructure interfacecitations
- 2016Engineering properties by long range symmetry propagation initiated at perovskite heterostructure interface
- 2015Co-rich ZnCoO nanoparticles embedded in wurtzite <tex>$Zn_{1-x}Co_{x}O$</tex> thin filmscitations
- 2014Crystal Structure and Luminescent Properties of R2-xEux(MoO4)(3) (R = Gd, Sm) Red Phosphorscitations
- 2014Influence of the structure on the properties of <tex>$Na_{x}Eu_{y}(MoO_{4})_{z}$</tex> red phosphorscitations
- 2012Artificial construction of the layered Ruddlesden–Popper Manganite La2Sr2Mn3O10by reflection high energy electron diffraction monitored pulsed laser deposition
- 2012Grain size tuning of nanocrystalline chemical vapor deposited diamond by continuous electrical bias growth: Experimental and theoretical studycitations
Places of action
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article
Artificial construction of the layered Ruddlesden–Popper Manganite La2Sr2Mn3O10by reflection high energy electron diffraction monitored pulsed laser deposition
Abstract
Pulsed laser deposition has been used to artificially construct the n = 3 Ruddlesden–Popper structure La2Sr2Mn3O10 in epitaxial thin film form by sequentially layering La1–xSrxMnO3 and SrO unit cells aided by in situ reflection high energy electron diffraction monitoring. The interval deposition technique was used to promote two-dimensional SrO growth. X-ray diffraction and cross-sectional transmission electron microscopy indicated that the trilayer structure had been formed. A site ordering was found to differ from that expected thermodynamically, with the smaller Sr2+ predominantly on the R site due to kinetic trapping of the deposited cation sequence. A dependence of the out-of-plane lattice parameter on growth pressure was interpreted as changing the oxygen content of the films. Magnetic and transport measurements on fully oxygenated films indicated a frustrated magnetic ground state characterized as a spin glass-like magnetic phase with the glass temperature Tg ≈ 34 K. The magnetic frustration has a clear in-plane (ab) magnetic anisotropy, which is maintained up to temperatures of 150 K. Density functional theory calculations suggest competing antiferromagnetic and ferromagnetic long-range orders, which are proposed as the origin of the low-temperature glassy state.