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article
Enthalpy of formation of ye’elimite and ternesite
Abstract
Calcium sulfoaluminate clinkers containing<br/>ye’elimite (Ca4Al6O12(SO4)) and ternesite (Ca5(SiO4)2<br/>SO4) are being widely investigated as components of calcium<br/>sulfoaluminate cement clinkers. These may become<br/>low energy replacements for Portland cement. Conditional<br/>thermodynamic data for ye’elimite and ternesite (enthalpy<br/>of formation) have been determined experimentally using a<br/>combination of techniques: isothermal conduction<br/>calorimetry, X-ray powder diffraction and thermogravimetric<br/>analysis. The enthalpies of formation of ye’elimite<br/>and ternesite at 25 C were determined to be - 8523 and<br/>- 5993 kJ mol-1, respectively.