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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Drewitt, James W. E.
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (12/12 displayed)
- 2022Boron incorporation in silicate melt
- 2022The glass transition and the non-Arrhenian viscosity of carbonate meltscitations
- 2022The glass transition and the non-Arrhenian viscosity of carbonate meltscitations
- 2022Boron incorporation in silicate melt:pressure-induced coordination changes and implications for B isotope fractionation
- 2021Structure of levitated Si-Ge melts studied by high-energy x-ray diffraction in combination with reverse Monte Carlo simulationscitations
- 2019Configurational constraints on glass formation in the liquid calcium aluminate systemcitations
- 2017Structure of rare-earth chalcogenide glasses by neutron and x-ray diffractioncitations
- 2016Neutron diffraction of calcium aluminosilicate glasses and meltscitations
- 2013Structure of (FexCa1-xO)(y)(SiO2)(1-y) liquids and glasses from high-energy x-ray diffractioncitations
- 2013Fragile glass - formers reveal their structural secrets
- 2013Structure of (FexCa1-xO)(y)(SiO2)(1-y) liquids and glasses from high-energy x-ray diffraction:Implications for the structure of natural basaltic magmascitations
- 2011Application of time resolved x-ray diffraction to study the solidification of glass-forming melts
Places of action
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article
Application of time resolved x-ray diffraction to study the solidification of glass-forming melts
Abstract
Using time resolved x-ray diffraction combined with aerodynamic levitation and CO2 laser heating, we have studied the structural evolution of the fragile glass-forming liquid CaAl2O4 during supercooling from the stable liquid phase to the cold glass below T-g. In particular, we followed the evolution of the structure factor S(Q) and of the corresponding pair distribution function g(r). The results show significant structural changes around 1.25 T-g indicating an increase in the degree of both intermediate-and short-range order occurring close to the dynamical crossover temperature. Experiments were carried out at several beamlines at various synchrotron sources and we show that the potential of third generation synchrotron beamlines is limited by the lack of efficient detectors for making time resolved measurements on disordered materials. In this paper, we present an overview of the advances performed in this area over the past 10 years pointing out the limitations and expectations for the near future.