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| Naji, M. |
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| Motta, Antonella |
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| Aletan, Dirar |
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| Mohamed, Tarek |
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| Ertürk, Emre |
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| Taccardi, Nicola |
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| Kononenko, Denys |
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| Petrov, R. H. | Madrid |
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| Alshaaer, Mazen | Brussels |
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| Bih, L. |
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| Casati, R. |
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| Muller, Hermance |
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| Kočí, Jan | Prague |
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| Šuljagić, Marija |
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| Kalteremidou, Kalliopi-Artemi | Brussels |
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| Azam, Siraj |
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| Ospanova, Alyiya |
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| Blanpain, Bart |
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| Ali, M. A. |
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| Popa, V. |
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| Rančić, M. |
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| Ollier, Nadège |
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| Azevedo, Nuno Monteiro |
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| Landes, Michael |
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| Rignanese, Gian-Marco |
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Kunther, Wolfgang
Technical University of Denmark
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (32/32 displayed)
- 2024Understanding the influence of cementitious blended mixtures on pyrrhotite oxidation and internal sulphate attack
- 2024Metals in Mine Tailings and Prospects for Use in Cementitious Materials
- 2024Mapping circular economy practices for steel, cement, glass, brick, insulation, and wood – A review for climate mitigation modelingcitations
- 2024Mapping circular economy practices for steel, cement, glass, brick, insulation, and wood – A review for climate mitigation modelingcitations
- 2024Performance of cementitious systems containing calcined clay in a chloride-rich environment : A review by TC-282 CCLcitations
- 2024Development of a Performance-Based Framework for Optimized Selection of Raw Materials to Mitigate ASR in Concrete
- 2024Advancements in Heavy Metal Stabilization
- 2024Oxidation of sulfides from secondary materials in cementitious binders as a function of environmental conditions
- 2024Electrodialytic extraction of copper, lead and zinc from sulfide mine tailings:Optimization of current density and operation time
- 2023Gypsum formation mechanisms and their contribution to crystallisation pressure in sulfate resistant hardened cement pastes during early external sulfate attack at low sulfate concentrationscitations
- 2023Phase changes in cementitious materials exposed to saline solutionscitations
- 2023Clay Brick Powder as Partial Cement Replacementcitations
- 2023Development of a Framework to Provide Concrete with a Low Carbon Footprint and Enhanced Resistance Against ASR-Induced Development
- 2023Thermodynamics of calcined clays used in cementitious binderscitations
- 2023Cementitious materials for oil-well abandonment and numerical simulations of cement durability at oil well conditions
- 2023Thermodynamics of calcined clays used in cementitious binders:origin to service life considerationscitations
- 2023Binary and Ternary Shale Binders with High Replacement Levels
- 2022Chloride binding in Portland composite cements containing metakaolin and silica fumecitations
- 2022Chloride binding in Portland composite cements containing metakaolin and silica fumecitations
- 2022Chloride binding in Portland composite cements containing metakaolin and silica fumecitations
- 2022Durability performance of binary and ternary blended cementitious systems with calcined claycitations
- 2022Heat of hydration vs. strength development of shale-limestone blended binders
- 2021Exploring sulphate resistance of coal mining waste blended cements through experiments and thermodynamic modellingcitations
- 2021Phase evolution and mechanical performance of an ettringite-based binder during hydrothermal agingcitations
- 2021Screening for key material parameters affecting early-age and mechanical properties of blended cementitious binders with mine tailingscitations
- 2021Impact of electrodialytic remediation of MSWI fly ash on hydration and mechanical properties of blends with Portland cementcitations
- 2019Sulfate resistance of calcined clay – limestone – Portland cementscitations
- 2019Chloride binding in blended binder systems: Importance of the structures of CSH gel
- 2019Chloride binding in blended binder systems: Importance of the structures of CSH gel
- 2017Influence of the Ca/Si ratio on the compressive strength of cementitious calcium-silicate-hydrate binderscitations
- 2015Durability of Portland Cement Blends Including Calcined Clay and Limestone: Interactions with Sulfate, Chloride and Carbonate Ionscitations
- 2013On the relevance of volume increase for the length changes of mortar bars in sulfate solutionscitations
Places of action
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document
Cementitious materials for oil-well abandonment and numerical simulations of cement durability at oil well conditions
Abstract
In this work, we investigate Portland cement hydration and durability at elevated temperatures of 60°C – 80°C and at pressures up to 300 bar in water and in artificial brine solutions that mimic the exposing environments of cement plugs used for abandonment of out-sourced off-shore oil wells. A principal aim is to follow the structural and compositional evolution of the C-S-H phase, and thus, solid-state <sup>27</sup>Al and <sup>29</sup>Si NMR are used as the main analytical tools. The NMR results indicate that hydration at high pressure (300 bar) has no significant impact on the C-S-H phases formed at 60 and 80 °C, however, it may retard the decomposition of ettringite and the AFm phases at 80 °C. Interestingly, the exposure of the hydrated cement paste to the laboratory-made brine solution significantly impacts the microstructure of the formed C-S-H product as a cross-linked C-S-H phase is formed at a high ratio of solution to solid. The samples are additionally cured in CO<sub>2</sub>-injected brine, and the effect of particle size on the carbonation degree is studied. The experimental phase assemblages from the investigations will be used in thermodynamic reactive-transport modeling to estimate the durability and physical properties of the hardened cement on a prolonged time scale.