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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Zia, Abdul Wasy
Heriot-Watt University
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (19/19 displayed)
- 2024Innovative Tin and hard carbon architecture for enhanced stability in lithium-ion battery anodescitations
- 2024Sputtered Hard Carbon for High-Performance Energy Storage Batteries
- 2024Designing Molybdenum Trioxide and Hard Carbon Architecture for Stable Lithium‐Ion Battery Anodescitations
- 2024Wear-resistant and adherent nanodiamond composite thin film for durable and sustainable silicon carbide mechanical seals.citations
- 2024Circular usage of waste cooking oil towards green electrical discharge machining process with lower carbon emissionscitations
- 2024Oxygen concentration – a governing parameter for microstructural tailoring of duplex AlCrSiON coatings for superior mechanical, tribological, and anti-corrosion performancecitations
- 2024Wear-resistant and Adherent Nanodiamond Composite Thin Film for Durable and Sustainable Silicon Carbide Mechanical Sealscitations
- 2024Role of scandium addition to microstructure, corrosion resistance, and mechanical properties of AA7085/ZrB2+Al2O3 compositescitations
- 2024Precision depth-controlled isolated silver nanoparticle-doped diamond-like carbon coatings with enhanced ion release, biocompatibility, and mechanical performancecitations
- 2023Soft diamond-like carbon coatings with superior biocompatibility for medical applicationscitations
- 2023Multi-layered Sn and Hard Carbon Architectures for Long-Term Stability and High-Capacity Lithium-Ion Battery Anodes
- 2023Role of biodegradable dielectrics toward tool wear and dimensional accuracy in Cu-mixed die sinking EDM of Inconel 600 for sustainable machiningcitations
- 2023Role of biodegradable dielectrics toward tool wear and dimensional accuracy in Cu-mixed die sinking EDM of Inconel 600 for sustainable machining
- 2023Advancing Lithium-Ion Battery Anodes: Novel Sn and Hard Carbon Architectures for Long-Term Stability and High Capacity
- 2022Disrupting biofilm and eradicating bacteria by Ag-Fe3O4@MoS2 MNPs nanocomposite carrying enzyme and antibioticscitations
- 2013Epitaxial growth of cerium oxide thin films by pulsed laser depositioncitations
- 2013Effect of Diamond like Carbon Coating Thickness on Stainless Steel Substrate
- 2012 Fracture Toughness of Plasma Coated Zirconia(ZrO₂)
- 2012Mechanical Characterization of PECVD coated Materials by Indentation Techniques and Finite Element Simulation
Places of action
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document
Advancing Lithium-Ion Battery Anodes: Novel Sn and Hard Carbon Architectures for Long-Term Stability and High Capacity
Abstract
Tin (Sn) is a promising candidate for lithium-ion batteries (LIBs) because of its high theoretical capacity, abundance, and low cost. However, Sn suffers from large volumetric expansion during charging and discharging causing cracking and degradation of the electrode material. Thus, development of new Sn based interfaces and architectures is crucial that can accommodate the volume changes and improve cyclic performance. In this study, we present the development of a novel Sn and hard carbon (h-carbon) architectures for LIB anodes, with a focus on improving their long-term stability and high capacity. The composite architectures is achieved through nano Physical Vapor Deposition (nano-PVD) technique by depositing Sn and hard carbon on Copper substrate at the room temperature and a high temperature (470 oC). Our results show that the Sn and h-carbon architectures exhibit significantly improved long-term cycling stability (> 94% coulombic efficiency after 25 cycles) and higher capacities reaching upto 915 mAh g-1 at 2nd cycle after SEI formation. The resultant microstructures especially at 400 oC created a multi-layer interface with Cu-Sn and h-carbon. The newly developed, so called soft (Cu-Sn) and a hard interface (h-Carbon) provides a cushion against volumetric expansion of Sn microstructures. These findings demonstrate the potential of Sn and hard carbon as promising anode materials for advancing the performance of LIBs.