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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Gao, Mei
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (20/20 displayed)
- 2024The first demonstration of entirely roll-to-roll fabricated perovskite solar cell modules under ambient room conditions
- 2024The first demonstration of entirely roll-to-roll fabricated perovskite solar cell modules under ambient room conditionscitations
- 2023Versatile Carbon Electrodes for Record Small, Large, Rigid, and Flexible Perovskite Solar Cells
- 2022Vacuum-free and solvent-free deposition of electrodes for roll-to-roll fabricated perovskite solar cellscitations
- 2022Effect of out-gassing from polymeric encapsulant materials on the lifetime of perovskite solar cellscitations
- 2021Can laminated carbon challenge gold? Towards universal, scalable and low-cost carbon electrodes for perovskite solar cellscitations
- 2020Develop Roll-to-Roll Compatible Process for Highly Efficient Thin Film Solar Cells (ICFPOE 2019)
- 2020Develop Roll-to-Roll Compatible Process for Highly Efficient Thin Film Solar Cells (ICFPOE 2019)
- 2020Develop Roll-to-Roll Compatible Process for Highly Efficient Thin Film Solar Cells (ICFPOE 2019)
- 2020Improving the Stability of Ambient-Processed SnO2-Based, Perovskite Solar Cells by UV-Treatment of the Sub-Cellscitations
- 2020Improving the Stability of Ambient processed, SnO2-Based, Perovskite Solar Cells by the UV-treatment of Sub-Cellscitations
- 2019Scalable, Stable, and Reproducible Roll-to-roll Processed Perovskite Solar Cells
- 2018Beyond fullerenes: Indacenodithienol-based organic charge transport layer towards upscaling of perovskite solar cellscitations
- 2018Reliability improvement of perovskite solar cells from roll-to-roll (R2R) continuous process
- 2018Manufacturing cost and market potential analysis of demonstrated roll-to roll perovskite photovoltaic cell processescitations
- 2017ITO-free flexible perovskite solar cells based on roll-to-roll, slot die coated silver nanowire electrodescitations
- 2017Printing-friendly sequential deposition via intra-additive approach for roll-to-roll production of perovskite solar cellscitations
- 2016Development of a high performance donor-acceptor conjugated polymer – synergy in materials and device optimizationcitations
- 2014Tailored donor-acceptor polymers with an A-D1-A-D2 structure: Controlling intermolecular interactions to enable enhanced polymer photovoltaic devicescitations
- 2014Organic Solar Cells Using a High-Molecular-Weight Benzodithiophene–Benzothiadiazole Copolymer with an Efficiency of 9.4%
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document
Scalable, Stable, and Reproducible Roll-to-roll Processed Perovskite Solar Cells
Abstract
The record efficiency of laboratory-scale perovskite solar cells has soared to 24%, bringing it on par with inorganic counterparts [1]. The challenge now is to develop an industry-compatible process for perovskite solar cell production that delivers dramatic cost and/or application benefits compared to existing products. A roll-to-roll manufacturing scheme with printing and coating deposition methods on flexible substrates under ambient environment conditions represents the ultimate low-cost and high-throughput production scheme. Perovskite absorber materials are exceptionally well-suited for such a processing scheme owing to their ease of incorporation into solution-based inks and low-temperature annealing requirements. Our progress on upscaling fabrication of planar p-i-n perovskite solar cells will be described in this presentation, including efficiency, stability, and reproducibility results, the latter being a key indicator for upscaling readiness of a given fabrication process. Firstly, a systematic optimization and evaluation of the device materials and structure was carried out using laboratory-scale cells fabricated by spin-coating on glass substrates using the anti-solvent method [2-3], with devices evaluated for efficiency, reproducibility, and stability. Secondly, a bench-top slot-die coater was employed to evaluate and optimize the perovskite absorber material deposition through a facile and reliable hot-deposition process [4]. The slot-die coating hot-deposition method was found to generate completely different perovskite morphology compared with the anti-solvent method, and devices were extensively characterized to unveil how these morphology differences affect opto-electronic properties. The processes developed in this work were then transferred to roll-to-roll coating on flexible substrates where all layers, except the electrodes, were slot-die coated. Scalability and process reliability were evaluated by utilising a flexible PET/ITO substrate patterned to give solar cells of three different areas (0.1 cm2, 1 cm2, 10 cm2) which are processed in-line during a single processing run. This enabled a comparison to be made between the roll-to-roll processed cells and the laboratory-scale benchmark devices, while also enabling evaluation of process reliability for further upscaling.References: [1] Best Research-Cell Efficiencies (NREL, accessed 25 July, 2019); https://www.nrel.gov/pv/assets/pdfs/best-research-cell-efficiencies.[2] Xiao, M., Huang, F., Huang, W., Dkhissi, Y., Zhu, Y., Etheridge, J., Gray-Weale, A., Bach, U., Cheng, Y., Spiccia, L. 2014, Angew. Chemie - Int. Ed., 126, p10056-59. [3] Jeon, N. J., Noh, J. H., Kim, Y. C., Yang, W. S.,Ryu, S., Seok, S. Il.,2014, Nat. Mater., 13, p897-903. [4] Vak, D., Hwang, K.,Faulks, A.,Jung, Y‐S., Clark, N.,Kim, D-Y., Wilson, G. J., Watkin, S. E., 2015, Advanced Energy Materials, 5.4, p1401539-46.