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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Zboril, Radek
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (15/15 displayed)
- 2022Interface Engineering of SRu-mC3N4 Heterostructures for Enhanced Electrochemical Hydrazine Oxidation Reactionscitations
- 2021The Hallmarks of Copper Single Atom Catalysts in Direct Alcohol Fuel Cells and Electrochemical CO<sub>2</sub> Fixationcitations
- 2021Single Co‐Atoms as Electrocatalysts for Efficient Hydrazine Oxidation Reactioncitations
- 2021The Hallmarks of Copper Single Atom Catalysts in Direct Alcohol Fuel Cells and Electrochemical CO2 Fixationcitations
- 2020Multi-Leg TiO2 Nanotube Photoelectrodes Modified by Platinized Cyanographene with Enhanced Photoelectrochemical Performancecitations
- 2020Graphitic Carbon Nitride–Nickel Catalyst: From Material Characterization to Efficient Ethanol Electrooxidationcitations
- 2018Unveiling BiVO4 nanorods as a novel anode material for high performance lithium ion capacitors: beyond intercalation strategiescitations
- 2018Unveiling BiVO4 nanorods as a novel anode material for high performance lithium ion capacitors: beyond intercalation strategiescitations
- 2018Ultrathin hierarchical porous carbon nanosheets for high-performance supercapacitors and redox electrolyte energy storagecitations
- 2018Ultrathin hierarchical porous carbon nanosheets for high-performance supercapacitors and redox electrolyte energy storagecitations
- 2018TiO2 Nanotubes on Transparent Substrates: Control of Film Microstructure and Photoelectrochemical Water Splitting Performancecitations
- 2018Unveiling BiVO4 nanorods as a novel anode material for high performance lithium ion capacitors : beyond intercalation strategiescitations
- 2018Ultrathin hierarchical porous carbon nanosheets for high‐performance supercapacitors and redox electrolyte energy storagecitations
- 2012Merging high doxorubicin loading with pronounced magnetic response and bio-repellent properties in hybrid drug nanocarrierscitations
- 2011The effect of surface modification on the fluorescence and morphology of CdSe nanoparticles embedded in a 3D phosphazene-based matrix: nanowire-like quantum dotscitations
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article
Interface Engineering of SRu-mC3N4 Heterostructures for Enhanced Electrochemical Hydrazine Oxidation Reactions
Abstract
<jats:p>Hydrazine oxidation in single-atom catalysts (SACs) could exploit the efficiency of metal atom utilization, which is a substitution for noble metal-based electrolysers that results in reduced overall cost. A well-established ruthenium single atom over mesoporous carbon nitride (SRu-mC3N4) catalyst is explored for the electro-oxidation of hydrazine as one of the model reactions for direct fuel cell reactions. The electrochemical activity observed with linear sweep voltammetry (LSV) confirmed that SRu-mC3N4 shows an ultra-low onset potential of 0.88 V vs. RHE, and with a current density of 10 mA/cm2 the observed potential was 1.19 V vs. RHE, compared with mesoporous carbon nitride (mC3N4) (1.77 V vs. RHE). Electrochemical impedance spectroscopy (EIS) and chronoamperometry (i-t) studies on SRu-mC3N4 show a smaller charge-transfer resistance (RCt) of 2950 Ω and long-term potential, as well as current stability of 50 h and 20 mA/cm2, respectively. Herein, an efficient and enhanced activity toward HzOR was demonstrated on SRu-mC3N4 from its synergistic platform over highly porous C3N4, possessing large and independent active sites, and improving the subsequent large-scale reaction.</jats:p>