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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Bdikin, Igor
University of Aveiro
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (8/8 displayed)
- 2022Sustainable Synthesis of Highly Biocompatible 2D Boron Nitride Nanosheetscitations
- 2021Nanoscale Piezoelectric Properties and Phase Separation in Pure and La-Doped BiFeO3 Films Prepared by Sol–Gel Methodcitations
- 2021Immobilised rGO/TiO2 Nanocomposite for Multi-Cycle Removal of Methylene Blue Dye from an Aqueous Mediumcitations
- 2021Graphene-Based TiO2 Nanocomposite for Photocatalytic Degradation of Dyes in Aqueous Solution under Solar-Like Radiationcitations
- 2017Growth, crystal structure, Hirshfeld surface, optical, piezoelectric, dielectric and mechanical properties of bis(L-asparaginium hydrogensquarate) single crystalcitations
- 2012Production and PFM characterization of barium titanate nanofiberscitations
- 2011Production of polar β-Glycine nanofibers with enhanced nonlinear optical and piezoelectric propertiescitations
- 2009Synthesis of polymer-based triglycine sulfate nanofibres by electrospinningcitations
Places of action
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article
Graphene-Based TiO2 Nanocomposite for Photocatalytic Degradation of Dyes in Aqueous Solution under Solar-Like Radiation
Abstract
<jats:p>This study presents a novel method for the development of TiO2/reduced graphene oxide (rGO) nanocomposites for photocatalytic degradation of dyes in an aqueous solution. The synergistic integration of rGO and TiO2, through the formation of Ti–O–C bonds, offers an interesting opportunity to design photocatalyst nanocomposite materials with the maximum absorption shift to the visible region of the spectra, where photodegradation can be activated not only with UV but also with the visible part of natural solar irradiation. TiO2@rGO nanocomposites with different content of rGO have been self-assembled by the hydrothermal method followed by calcination treatment. The morphological and structural analysis of the synthesized photocatalysts was performed by FTIR, XRD, XPS, UV-Vis DRS, SEM/EDX, and Raman spectroscopy. The effectiveness of the synthesized nanocomposites as photocatalysts was examined through the photodegradation of methylene blue (MB) and rhodamine B (RhB) dye under artificial solar-like radiation. The influence of rGO concentration (5 and 15 wt.%) on TiO2 performance for photodegradation of the different dyes was monitored by UV-Vis spectroscopy. The obtained results showed that the synthesized TiO2@rGO nanocomposites significantly increased the decomposition of RhB and MB compared to the synthesized TiO2 photocatalyst. Furthermore, TiO2@rGO nanocomposite with high contents of rGO (15 wt.%) presented an improved performance in photodegradation of MB (98.1%) and RhB (99.8%) after 120 min of exposition to solar-like radiation. These results could be mainly attributed to the decrease of the bandgap of synthesized TiO2@rGO nanocomposites with the increased contents of rGO. Energy gap (Eg) values of nanocomposites are 2.71 eV and 3.03 eV, when pure TiO2 particles have 3.15 eV. These results show the potential of graphene-based TiO2 nanocomposite to be explored as a highly efficient solar light-driven photocatalyst for water purification.</jats:p>