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| Naji, M. |
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| Motta, Antonella |
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| Aletan, Dirar |
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| Mohamed, Tarek |
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| Ertürk, Emre |
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| Taccardi, Nicola |
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| Kononenko, Denys |
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| Petrov, R. H. | Madrid |
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| Alshaaer, Mazen | Brussels |
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| Bih, L. |
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| Casati, R. |
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| Muller, Hermance |
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| Kočí, Jan | Prague |
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| Šuljagić, Marija |
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| Kalteremidou, Kalliopi-Artemi | Brussels |
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| Azam, Siraj |
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| Ospanova, Alyiya |
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| Blanpain, Bart |
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| Ali, M. A. |
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| Popa, V. |
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| Rančić, M. |
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| Ollier, Nadège |
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| Azevedo, Nuno Monteiro |
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| Landes, Michael |
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| Rignanese, Gian-Marco |
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Delport, Géraud
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (16/16 displayed)
- 2021Rational Passivation of Sulfur Vacancy Defects in Two-Dimensional Transition Metal Dichalcogenides.
- 2021Local Energy Landscape Drives Long-Range Exciton Diffusion in Two-Dimensional Halide Perovskite Semiconductors.
- 2020Mechanistic Insight to the Chemical Treatments of Monolayer Transition Metal Disulfides for Photoluminescence Enhancement
- 2020Structural and spectroscopic studies of a nanostructured silicon-perovskite interface.
- 2019Imaging carrier transport properties in halide perovskites using time-resolved optical microscopy
- 2019Room-Temperature Cavity Polaritons with 3D Hybrid Perovskite: Toward Large-Surface Polaritonic Devicescitations
- 2019Enhancing Photoluminescence and Mobilities in WS2 Monolayers with Oleic Acid Ligands.
- 2018Using a confocal PL microscope to correlate the PL and structural properties of 2D-layered perovskites crystals and thin films
- 2018Time-resolved microphotoluminescence study of 2D layered hybrid perovskites crystals. Correlation between the structural and optical properties.
- 2018Time-resolved microphotoluminescence study of 2D layered hybrid perovskites crystals. Correlation between the structural and optical properties.
- 2018Micro-photoluminescence study of 2D-layered hybrid perovskite monocrystalline thin films. Correlation between the structural and optoelectronics properties
- 2018Micro-photoluminescence study of 2D-layered hybrid perovskite monocrystalline thin films. Correlation between the structural and optoelectronics properties
- 2018Exciton dynamics in 2D layered Hybrid Perovskites Crystals
- 2018Exciton dynamics in 2D layered Hybrid Perovskites Crystals
- 2017Micro-photoluminescence study of halide perovskites monocrystalline films. Correlation between the structural and optoelectronics properties.
- 2017Photophysics of self-assembled luminophore-perovskite systems
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article
Local Energy Landscape Drives Long-Range Exciton Diffusion in Two-Dimensional Halide Perovskite Semiconductors.
Abstract
Halide perovskites are versatile semiconductors with applications including photovoltaics and light-emitting devices, having modular optoelectronic properties realizable through composition and dimensionality tuning. Layered Ruddlesden-Popper perovskites are particularly interesting due to their unique 2D character and charge carrier dynamics. However, long-range energy transport through exciton diffusion in these materials is not understood or realized. Here, local time-resolved luminescence mapping techniques are employed to visualize exciton transport in exfoliated flakes of the BA2MAn-1PbnI3n+1 perovskite family. Two distinct transport regimes are uncovered, depending on the temperature range. Above 100 K, diffusion is mediated by thermally activated hopping processes between localized states. At lower temperatures, a nonuniform energy landscape emerges in which transport is dominated by downhill energy transfer to lower-energy states, leading to long-range transport over hundreds of nanometers. Efficient, long-range, and switchable downhill transfer offers exciting possibilities for controlled directional long-range transport in these 2D materials for new applications. ; The authors acknowledge the European Research Council (ERC) under the European Union’s Horizon 2020 research and innovation program (HYPERION, Grant Agreement Number 756962). SDS acknowledges funding from the Royal Society and Tata Group (UF150033). GD acknowledges the Royal Society for funding through a Newton International Fellowship. GD and SDS acknowledge the UK Engineering and Physical Sciences Research Council (EPSRC) under grant reference EP/R023980/1. A.B. acknowledges a Robert Gardiner Scholarship and funding from Christ’s College, Cambridge. K.G. acknowledges support from the Polish Ministry of Science and Higher Education within the Mobilnosc Plus program (GrantNo.1603/MOB/V/2017/0). The authors thank Niall Goulding and Rachel Bothwell for valuable discussions.