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Anton, Josef
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article
Surface Modification of a n-Si(111) Electrode through Aldehyde Grafting and Subsequent Metallization: Theory and Experiment
Abstract
<jats:title>Abstract</jats:title><jats:p>Motivated by our previous studies on metallic substrates, in the present work we addressed the functionalization and the subsequent metallization of a hydrogen-terminated <jats:italic>n</jats:italic>-Si(111) electrode. DFT provides atomistic insights on the grafting mechanism of 4-pyridinecarboxaldehyde (C<jats:sub>6</jats:sub>H<jats:sub>5</jats:sub>NO) what encouraged electrochemical investigations, <jats:italic>i. e.</jats:italic> cyclic voltammetry and <jats:italic>in-situ</jats:italic> STM, combined with XPS measurements which together provide evidence for a successful transfer of the so far obtained knowledge from metal single crystal to semiconductor surfaces.</jats:p>