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Muts, Ihor
Lviv University
in Cooperation with on an Cooperation-Score of 37%
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article
Equiatomic indides REIrIn (RE=La, Pr, Nd, Er–Yb) – Crystal and electronic structure
Abstract
<jats:title>Abstract</jats:title><jats:p>The equiatomic rare earth iridium indides<jats:italic>RE</jats:italic>IrIn (<jats:italic>RE</jats:italic>=La, Pr, Nd, Er–Yb) were synthesized by reaction of the elements in induction or muffle furnaces and were characterized through X-ray powder patterns. The structures of LaIr<jats:sub>0.86</jats:sub>In<jats:sub>1.14</jats:sub>, PrIr<jats:sub>0.89</jats:sub>In<jats:sub>1.11</jats:sub>, NdIr<jats:sub>0.94</jats:sub>In<jats:sub>1.06</jats:sub>, ErIrIn (all ZrNiAl type,<jats:italic>P</jats:italic>6̅2<jats:italic>m</jats:italic>), and YbIrIn (TiNiSi type,<jats:italic>Pnma</jats:italic>) were refined from single crystal X-ray diffractometer data. Refinements of the occupancy parameters revealed small degrees of solid solutions with indium substitution on the iridium sites. Chemical bonding analyses and electronic structure calculations indicate the dominance of metallic bonding in addition to partial ionic interactions between the cations and polyanions, as well as covalent contributions between the indium and iridium atoms.</jats:p>