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| Azevedo, Nuno Monteiro |
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Kegler, Philip
in Cooperation with on an Cooperation-Score of 37%
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article
New insights into phosphate based materials for the immobilisation of actinides
Abstract
<jats:title>Abstract</jats:title><jats:p>This paper focuses on major phosphate-based ceramic materials relevant for the immobilisation of Pu, minor actinides, fission and activation products. Key points addressed include the recent progress regarding synthesis methods, the formation of solid solutions by structural incorporation of actinides or their non-radioactive surrogates and waste form fabrication by advanced sintering techniques. Particular attention is paid to the properties that govern the long-term stability of the waste forms under conditions relevant to geological disposal. The paper highlights the benefits gained from synergies of state-of-the-art experimental approaches and advanced atomistic modeling tools for addressing properties and stability of</jats:p>