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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Sahraoui, Bouchta
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (26/26 displayed)
- 2024Synthesis, nanocrystalline morphology, lattice dynamics and nonlinear optics of mesoporous SiO2&LiNbO3 nanocomposite
- 2024Synthesis, nanocrystalline morphology, lattice dynamics and nonlinear optics of mesoporous SiO2&LiNbO3 nanocomposite
- 2023Second harmonic generation on crystalline organic nanoclusters under extreme nanoconfinement in functionalized silica–benzil compositescitations
- 2022Tetrabutylammonium (TBA)-Doped Methylammonium Lead Iodide: High Quality and Stable Perovskite Thin Filmscitations
- 2022Correlation between Nonlinear Optical Effects and Structural Features of Aurone-Based Methacrylic Polymeric Thin Filmscitations
- 2021Anisotropic confinement of chromophores induces second-order nonlinear optics in a nanoporous photonic metamaterialcitations
- 2020Effect of Ar Gas Pressure on LSPR Property of Au Nanoparticles: Comparison of Experimental and Theoretical Studies.citations
- 2017Spin-coated nickel doped cadmium sulfide thin films for third harmonic generation applicationscitations
- 2016Linear and Nonlinear Optical properties of ZnO Thin Films deposited by Pulsed Laser Depositiocitations
- 2016Electrical and structural analysis of xPbO-(1-x)B 2 O 3 (0.3≤ x≤ 0.9) glassescitations
- 2015Optical characteristics of a-Si: H layers deposited by PACVD at various temperaturescitations
- 2015Multimodal Vibration Damping of a Smart Beam Structure using Modal SSDI-Max Technique
- 2015Nonlinear optical properties of poly (methyl methacrylate) thin films doped with Bixa Orellana dyecitations
- 2014Dye-sensitized solar cells with PVA–KI–EC–PC gel electrolytescitations
- 2014Impact of annealing process on stacking orientations and second order nonlinear optical properties of metallophthalocyanine thin films and nanostructurescitations
- 2013Investigation of superfast deposition of metal oxide and Diamond-Like Carbon thin films by nanosecond Ytterbium (Yb+) fiber lasercitations
- 2012Novel Styrylquinolinium Dye Thin Films Deposited by Pulsed Laser Deposition for Nonlinear Optical Applicationscitations
- 2012Mechanical characterization of an electrostrictive polymer for actuation and energy harvestingcitations
- 2012Nonlinear photonics properties of porphyrins nanocomposites and self-assembled porphyrinscitations
- 2012Alkynyl-ruthenium based azo-organometallics : thermal evolution of thin films microstructurecitations
- 2011Non-linear optical and electrical properties of ZnO doped Ni Thin Films obtained using spray ultrasonic techniquecitations
- 2010Correlation between structural studies and third order NLO properties of selected new quinolinium semi-organic compoundscitations
- 2009Linear and nonlinear optical properties of ZnO/PMMA nanocomposite filmscitations
- 2009Linear and nonlinear optical properties of the CdSe nanocrystals embedded in PMMA matrix
- 2007Manifestation of electron-phonon interactions in IR-induced second harmonic generation in a sulphide glass-ceramic with β-GeS2 microcrystallitescitations
- 2002Quasi-phase-matched gratings printed by all-optical poling in polymer filmscitations
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article
Anisotropic confinement of chromophores induces second-order nonlinear optics in a nanoporous photonic metamaterial
Abstract
Second-order nonlinear optics is the base for a large variety of devices aimed at the active manipulation of light. However, physical principles restrict its occurrence to non-centrosymmetric, anisotropic matter. This significantly limits the number of base materials exhibiting nonlinear optics. Here, we show that embedding chromophores in an array of conical channels 13 nm across in monolithic silica results in mesoscopic anisotropic matter and thus in a hybrid material showing second-harmonic generation. This nonlinear optics is compared to the one achieved in corona-poled polymer films containing the identical chromophores. It originates in the confinement-induced orientational order of the elongated guest molecules in the nanochannels. This leads to a non-centrosymmetric dipolar order and hence to a nonlinear light–matter interaction on the sub-wavelength, single-pore scale. Our study demonstrates that the advent of large-scale, self-organized nanoporosity in monolithic solids along with the confinement-controllable orientational order of chromophores at the single-pore scale provides a reliable and accessible tool to design materials with a nonlinear meta-optics.