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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Cox, Joel D.
University of Southern Denmark
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (15/15 displayed)
- 2024Quantum-mechanical effects in photoluminescence from thin crystalline gold filmscitations
- 2024Quantum-mechanical effects in photoluminescence from thin crystalline gold filmscitations
- 2024Nonlocal effects in plasmon-emitter interactionscitations
- 2023Nonlinear Plasmonics in Nanostructured Phosphorenecitations
- 2023Nonlinear Plasmonics in Nanostructured Phosphorenecitations
- 2023Photoluminescence from Ultrathin Monocrystalline Gold Flakes
- 2023Photoluminescence from Ultrathin Monocrystalline Gold Flakes
- 2021Nonlinear plasmonic response in atomically thin metal filmscitations
- 2021Nonlinear plasmonic response in atomically thin metal filmscitations
- 2021Anisotropic second-harmonic generation from monocrystalline gold flakescitations
- 2021Anisotropic second-harmonic generation from monocrystalline gold flakescitations
- 2020Strong-field-driven dynamics and high-harmonic generation in interacting one dimensional systemscitations
- 2020Strong-field-driven dynamics and high-harmonic generation in interacting one dimensional systemscitations
- 2019Quantum effects in the acoustic plasmons of atomically thin heterostructurescitations
- 2019Quantum effects in the acoustic plasmons of atomically thin heterostructurescitations
Places of action
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article
Anisotropic second-harmonic generation from monocrystalline gold flakes
Abstract
Noble metals with well-defined crystallographic orientation constitute an appealing class of materials for controlling light–matter interactions on the nanoscale. Nonlinear optical processes, being particularly sensitive to anisotropy, are a natural and versatile probe of crystallinity in nano-optical devices. Here we study the nonlinear optical response of monocrystalline gold flakes, revealing a polarization dependence in second-harmonic generation from the {111} surface that is markedly absent in polycrystalline films. Our findings confirm that second-harmonic microscopy is a robust and non-destructive method for probing the crystallographic orientation of gold, and can serve as a guideline for enhancing nonlinear response in plasmonic systems.