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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Boroviks, Sergejs
École Polytechnique Fédérale de Lausanne
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (9/9 displayed)
- 2023Photon superbunching in cathodoluminescence of excitons in WS 2 monolayercitations
- 2023Photon superbunching in cathodoluminescence of excitons in WS2 monolayercitations
- 2023Photon superbunching in cathodoluminescence of excitons in WS2 monolayercitations
- 2022Extremely confined gap plasmon modescitations
- 2022Extremely confined gap plasmon modes:when nonlocality matterscitations
- 2022Low-loss anisotropic image polaritons in van der waals crystal α-MoO 3citations
- 2021Anisotropic second-harmonic generation from monocrystalline gold flakescitations
- 2021Anisotropic second-harmonic generation from monocrystalline gold flakescitations
- 2020Linear and Nonlinear Plasmonics with Monocrystalline Gold Flakes
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article
Anisotropic second-harmonic generation from monocrystalline gold flakes
Abstract
Noble metals with well-defined crystallographic orientation constitute an appealing class of materials for controlling light–matter interactions on the nanoscale. Nonlinear optical processes, being particularly sensitive to anisotropy, are a natural and versatile probe of crystallinity in nano-optical devices. Here we study the nonlinear optical response of monocrystalline gold flakes, revealing a polarization dependence in second-harmonic generation from the {111} surface that is markedly absent in polycrystalline films. Our findings confirm that second-harmonic microscopy is a robust and non-destructive method for probing the crystallographic orientation of gold, and can serve as a guideline for enhancing nonlinear response in plasmonic systems.