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Gubbins, Keith E.
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article
Melting of mixtures in silica nanopores
Abstract
<p>We report experimental measurements of the melting of mixtures confined in nanoporous materials. Dielectric relaxation spectroscopy (DRS) was used to determine the solid-liquid phase diagram of bromobenzene/carbon tetrachloride (C<sub>6</sub>H<sub>5</sub>Br/CCl<sub>4</sub>) mixtures confined in controlled pore glasses (CPGs) with an average pore diameter H = 7.5 nm. Our results show that the phase diagram of the confined mixture is of the same type as that for the bulk, but the solid-liquid coexistence lines are located at different temperatures. These results are compared with those previously obtained for CCl<sub>4</sub>/C<sub>6</sub>H<sub>6</sub> mixtures in activated carbon fibers (ACFs). © 2009 IUPAC,.</p>