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Hara, Takayoshi
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article
In Situ Generation of Catalytically Active Cu0 Species Derived from Cu-Al Layered Double Hydroxides for Acceptorless Alcohol Dehydrogenation
Abstract
<jats:title>Abstract</jats:title><jats:p>A CuO-CuAl2O4 nanocomposite (CuAl NC) synthesized by high temperature calcination of Cu-Al layered double hydroxides (CuAl LDHs) acted as an effective heterogeneous catalyst for acceptorless dehydrogenation of various alcohols. The catalytically active Cu0 species was formed by in situ reduction with alcohol. The catalytic activity strongly depended on the Cu/Al ratio in preparation and calcination temperature. The synthesized catalyst was reusable without loss of its high activity and selectivity.</jats:p>