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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Knapp, Michael
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (26/26 displayed)
- 2024Understanding the Electrochemical Reaction Mechanism of the Co/Ni Free Layered Cathode Material P2–Na$_{2/3}$Mn$_{7/12}$Fe$_{1/3}$Ti$_{1/12}$O$_{2}$ for Sodium-Ion Batteries
- 2024Understanding the Electrochemical Reaction Mechanism of the Co/Ni Free Layered Cathode Material P2–Na$_{2/3}$Mn$_{7/12}$Fe$_{1/3}$Ti$_{1/12}$O$_2$ for Sodium-Ion Batteriescitations
- 2023In situ neutron diffraction for analysing complex coarse‐grained functional materialscitations
- 2023In situ neutron diffraction for analysing complex coarse-grained functional materials
- 2022Methods—Spatially Resolved Diffraction Study of the Uniformity of a Li-Ion Pouch Cellcitations
- 2022Unveiling the Electrochemical Mechanism of High-Capacity Negative Electrode Model-System BiFeO 3 in Sodium-Ion Batteries: An In Operando XAS Investigationcitations
- 2021Garnet to hydrogarnet: effect of post synthesis treatment on cation substituted LLZO solid electrolyte and its effect on Li ion conductivitycitations
- 2021Investigation of capacity fade for 18650-type lithium-ion batteries cycled in different state of charge (SoC) rangescitations
- 2020Fatigue in High-Energy Commercial Li Batteries while Cycling at Standard Conditions:An in Situ Neutron Powder Diffraction Studycitations
- 2020Mechanochemical synthesis of amorphous and crystalline $Na_{2}P_{2}S_{6}$ – elucidation of local structural changes by X-ray total scattering and NMRcitations
- 2020Lithium-ion (de)intercalation mechanism in core-shell layered Li(Ni,Co,Mn)O2 cathode materialscitations
- 2019Amorphous versus Crystalline $Li_3PS_{4}$: Local Structural Changes during Synthesis and Li Ion Mobilitycitations
- 2018Energy research with neutrons (ErwiN) and installation of a fast neutron powder diffraction option at the MLZ, Germanycitations
- 2018(De)Lithiation Mechanism of Hierarchically Layered LiNi$_{1/3}$Co$_{1/3}$Mn$_{1/3}$O$_{2}$ Cathodes during High-Voltage Cyclingcitations
- 2017Local Structures and Li Ion Dynamics in a $mathrm{Li_{10}SnP_{2}S_{12}}$ -Based Composite Observed by Multinuclear Solid-State NMR Spectroscopycitations
- 2017Average vs. local structure and composition-property phase diagram of $mathrm{K_{0.5}Na_{0.5}NbO_{3}-Bi_{½}Na_{½}TiO_{3}}$ systemcitations
- 2017Average vs. local structure and composition-property phase diagram of K 0.5 Na 0.5 NbO 3 -Bi ½ Na ½ TiO 3 systemcitations
- 2016Microwave synthesis of high-quality and uniform 4 nm ZnFe₂O₄ nanocrystals for application in energy storage and nanomagnetics
- 2016The phase diagram of $mathrm{K_{0.5}Na_{0.5}NbO_{3}–Bi_{1/2}Na_{1/2}TiO_{3}}$citations
- 2016Effect of internal current flow during the sintering of zirconium diboride by field assisted sintering technology ; Effekt des internen Stromflusses während der Sinterung von ZrB2 by FAST/SPScitations
- 2016Structure and dielectric dispersion in cubic-like $mathrm{0.5K_{0.5}Na_{0.5}NbO_{3}-0.5Na_{1/2}Bi_{1/2}TiO_{3}}$ ceramiccitations
- 2014Structural Contribution to the Ferroelectric Fatigue in Lead Zirconate Titanate (PZT) Ceramicscitations
- 2013Structural and electrochemical studies of the Li-In alloys
- 2008Nanodomains in morphotropic lead zirconate titanate ceramics : On the origin of the strong piezoelectric effectcitations
- 2007Nanodomains in morphotropic lead zirconate titanate ceramics : On the origin of the strong piezoelectric effectcitations
- 2006Iron-oxygen vacancy defect association in polycrystalline iron-modified PbZrO3 antiferroelectrics: Multifrequency electron paramagnetic resonance and Newman superposition model analysis
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article
Methods—Spatially Resolved Diffraction Study of the Uniformity of a Li-Ion Pouch Cell
Abstract
A lab-made, multilayered Li-ion battery pouch cell is investigated using in-operando neutron powder diffraction (NPD) and spatially resolved powder X-ray diffraction (SR-PXRD) with the aim of investigating how to compare the information obtained from the two complementary techniques on a cell type with a complicated geometry for diffraction. The work focusses on the anode and cathode lithiation as obtained from the LiC6/LiC12 weight ratio and the NMC111 c/a-ratio, respectively. Neutron powder diffractograms of a sufficient quality for Rietveld refinement are measured using a rotation stage to minimize geometrical effects. Using SR-PXRD, the cell is shown to be non-uniform in its anode and cathode lithiation, with the edges of the cell being less lithiated/delithiated than the center in the fully charged state. The non-uniformity is more pronounced for high charging current than low charging current. The averaged SR-PXRD data is found to match the bulk NPD data well. This is encouraging as it seems to allow comparisons between studies using either of these complementary techniques. This work will also serve as a benchmark for our future studies on pouch cells with novel non-commercial cathode and/or anode materials.