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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Praus, Petr
Charles University
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (10/10 displayed)
- 2021Tailoring the stoichiometry of C 3 N 4 nanosheets under electron beam irradiationcitations
- 2021Tailoring the stoichiometry of C3N4 nanosheets under electron beam irradiation
- 2021Tailoring the stoichiometry of C3N4 nanosheets under electron beam irradiationcitations
- 2020Deciphering the effect of traps on electronic charge transport properties of methylammonium lead tribromide perovskitecitations
- 2014ZnS/MMT nanocomposites : the effect of ZnS loading in MMT on the photocatalytic reduction of carbon dioxidecitations
- 2014Photocatalytic and photochemical decomposition of N2O on ZnS-MMT Catalystcitations
- 2013Nanocomposite of montmorillonite and silver nanoparticles: Characterization and application in catalytic reduction of 4-nitrophenolcitations
- 2011CdS nanoparticles deposited on montmorillonite: preparation, characterization and application for photoreduction of carbon dioxidecitations
- 2010Preparation and characterization of ZnS nanoparticles deposited on montmorillonitecitations
- 2010Adsorption of zinc and copper ions on natural and ethylenediamine modified montmorillonite
Places of action
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article
Deciphering the effect of traps on electronic charge transport properties of methylammonium lead tribromide perovskite
Abstract
<jats:p>Halide perovskites have undergone remarkable developments as highly efficient optoelectronic materials for a variety of applications. Several studies indicated the critical role of defects on the performance of perovskite devices. However, the parameters of defects and their interplay with free charge carriers remain unclear. In this study, we explored the dynamics of free holes in methylammonium lead tribromide (MAPbBr<jats:sub>3</jats:sub>) single crystals using the time-of-flight (ToF) current spectroscopy. By combining ToF spectroscopy and Monte Carlo simulation, three energy states were detected in the bandgap of MAPbBr<jats:sub>3</jats:sub>. In addition, we found the trapping and detrapping rates of free holes ranging from a few microseconds to hundreds of microseconds. Contrary to previous studies, we revealed a strong detrapping activity of traps. We showed that these traps substantially affect the transport properties of MAPbBr<jats:sub>3</jats:sub>, including mobility and mobility-lifetime product. Our results provide an insight on charge transport properties of perovskite semiconductors.</jats:p>