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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Lagoudakis, Pavlos
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Publications (7/7 displayed)
- 2022Enhanced coupling between ballistic exciton-polariton condensates through tailored pumpingcitations
- 2022FAPbBr3 perovskite quantum dots as a multifunctional luminescent-downshifting passivation layer for GaAs solar cellscitations
- 2021Realizing optical persistent spin helix and stern-gerlach deflection in an anisotropic liquid crystal microcavitycitations
- 2021Exciton energy spectra in polyyne chainscitations
- 2020Correlating Phase Behavior with Photophysical Properties in Mixed‐Cation Mixed‐Halide Perovskite Thin Filmscitations
- 2019A few-minute synthesis of CsPbBr3 nanolasers with a high quality factor by spraying at ambient conditionscitations
- 2013Single-mode tunable laser emission in the single-exciton regime from colloidal nanocrystalscitations
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article
Exciton energy spectra in polyyne chains
Abstract
Recently, we have experimentally observed signatures of sharp exciton peaks in the photoluminescence spectra of bundles of monoatomic carbon chains stabilized by gold nanoparticles and deposited on a glass substrate. Here we estimate the characteristic energies of excitonic transitions in this complex quasi-one-dimensional nanosystem with use of the variational method. We show that the characteristic energy scale for the experimentally observed excitonic fine structure is governed by the interplay between the hopping energy in a Van der Waals quasicrystal formed by parallel carbon chains, neutral-charged exciton splitting, and positive-negative trion splitting. These three characteristic energies are an order of magnitude lower than the direct exciton binding energy.