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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Como, Enrico Da
University of Bath
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (6/6 displayed)
- 2023Exploring the Charge Density Wave Phase of 1T-TaSe2citations
- 2020Excitonic and lattice contributions to the charge density wave in 1T-TiSe2 revealed by a phonon bottleneckcitations
- 2019Quantitative resonant soft x-ray reflectivity from an organic semiconductor single crystalcitations
- 2013Silica Nanoparticles for Enhanced Carrier Transport in Polymer-Based Short Channel Transistorscitations
- 2012The Effect of Ageing on Exciton Dynamics, Charge Separation, and Recombination in P3HT/PCBM Photovoltaic Blendscitations
- 2012The effect of ageing on exciton dynamics, charge separation, and recombination in P3HT/PCBM photovoltaic blendscitations
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article
Exploring the Charge Density Wave Phase of 1T-TaSe2
Abstract
<p>1T-TaSe2 is widely believed to host a Mott metal-insulator transition in the charge density wave (CDW) phase according to the spectroscopic observation of a band gap that extends across all momentum space. Previous investigations inferred that the occurrence of the Mott phase is limited to the surface only of bulk specimens, but recent analysis on thin samples revealed that the Mott-like behavior, observed in the monolayer, is rapidly suppressed with increasing thickness. Here, we report combined time- and angle-resolved photoemission spectroscopy and theoretical investigations of the electronic structure of 1T-TaSe2. Our experimental results confirm the existence of a state above EF, previously ascribed to the upper Hubbard band, and an overall band gap of ∼0.7 eV at Γ¯. However, supported by density functional theory calculations, we demonstrate that the origin of this state and the gap rests on band structure modifications induced by the CDW phase alone, without the need for Mott correlation effects.</p>