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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Grinenko, Vadim
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (11/11 displayed)
- 2018Dynamic magnetism in the disordered hexagonal double perovskite BaTi$_{1/2}$Mn$_{1/2}$O$_{3}$citations
- 2018Universal scaling behavior of the upper critical field in strained FeSe0.7Te0.3 thin filmscitations
- 2017The influence of the in-plane lattice constant on the superconducting transition temperature of FeSe0.7Te0.3 thin films
- 2016Hall-plot of the phase diagram for Ba(Fe₁₋ₓCoₓ)₂As₂
- 2016Hall-plot of the phase diagram for Ba(Fe1-xCox)2As2citations
- 2016Hall-plot of the phase diagram for Ba(Fe1−xCox)2As2
- 2015High field superconducting properties of Ba(Fe1-xCox)2As2 thin films
- 2015High field superconducting properties of Ba(Fe₁₋ₓCoₓ)₂As₂ thin filmscitations
- 2013Strain induced superconductivity in the parent compound BaFe2As2citations
- 2013Specific heat of Ca$_{0.32}$Na$_{0.68}$Fe$_2$As$_2$ single crystals: unconventional s$_pm$ multi-band superconductivity with intermediate repulsive interband coupling and sizable attractive intraband couplingscitations
- 2011As-vacancies, local moments, and Pauli limiting in LaO_0.9F_0.1FeAs_(1-delta) superconductorscitations
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document
As-vacancies, local moments, and Pauli limiting in LaO_0.9F_0.1FeAs_(1-delta) superconductors
Abstract
We report magnetization measurements of As-deficient LaO_0.9F_0.1FeAs_1-delta (delta about 0.06) samples with improved superconducting properties as compared with As-stoichiometric optimally doped La-1111 samples. In this As-deficient system with almost homogeneously distributed As-vacancies (AV), as suggested by the (75)As-nuclear quadrupole resonance (NQR) measurements,we observe a strong enhancement of the spin-susceptibility by a factor of 3-7. This observation is attributed to the presence of an electronically localized state around each AV, carrying a magnetic moment of about 3.2 mu_Bohr per AV or 0.8 mu_Bohr/Fe atom. From theoretical considerations we find that the formation of a local moment on neighboring iron sites of an AV sets in when the local Coulomb interaction exceeds a critical value of about 1.0 eV in the dilute limit. Its estimated value amounts to ~ 2.5 eV and implies an upper bound of ~ 2 eV for the Coulomb repulsion at Fe sites beyond the first neighbor-shell of an AV. Electronic correlations are thus moderate/weak in doped La-1111. The strongly enhanced spin susceptibility is responsible for the Pauli limiting behavior of the superconductivity that we observe in As-deficient LaO_0.9F_0.1FeAs_1-delta. In contrast, no Pauli limiting behavior is found for the optimally doped, As-stoichiometric LaO_0.9F_0.1FeAs superconductor in accord with its low spin susceptibility. ; Comment: 11 pages, 9 figures