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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Minár, J.
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Topics
Publications (15/15 displayed)
- 2023Are high-energy photoemission final states free-electron-like?
- 2023High-energy photoemission final states beyond the free-electron approximation
- 2022Band dispersion within pristine InBi crystal
- 2020Néel Vector Induced Manipulation of Valence States in the Collinear Antiferromagnet Mn$_2$ Aucitations
- 2018Distinctive Picosecond Spin Polarization Dynamics in Bulk Half Metalscitations
- 2017Spin-filtered time-of-flight $k$-space microscopy of Ir – Towards the “complete” photoemission experimentcitations
- 2016Disentangling bulk and surface Rashba effects in ferroelectric ${alpha}$-GeTecitations
- 2016Entanglement and manipulation of the magnetic and spin-orbit order in multiferroic Rashba semiconductorscitations
- 2015Monitoring surface resonances on Co2MnSi (100) by spin-resolved photoelectron spectroscopycitations
- 2014Correlation effects in fcc-Fe.sub.x./sub.Ni.sub.1-x./sub. alloys investigated by means of the KKR-CPAcitations
- 2014Direct observation of half-metallicity in the Heusler compound Co2MnSicitations
- 2014The Quest for and Demonstration of direct Experimental Evidence for half Metallicity in Heusler Compounds
- 2011Hard x-ray photoemission study of near-Heusler FexSi 1-x alloyscitations
- 2011Enhanced iron magnetic moment in the ThFe11C2 intermetallic compoundcitations
- 2010Theory of relativistic photoemission for correlated magnetic alloys: LSDA + DMFT study of the electronic structure of Ni $_{x}$ Pd $_{1 − x}$citations
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article
Hard x-ray photoemission study of near-Heusler FexSi 1-x alloys
Abstract
<p>The structural and electronic properties of epitaxial and amorphous Fe <sub>x</sub>Si<sub>1-x</sub> alloys with x = 0.72 and 0.67 near the binary Heusler composition of x = 0.75 were determined using hard x-ray photoelectron spectroscopy (HXPS). By performing the measurements at a photon energy of 5950.3 eV, the bulk-sensitivity of the measurement is enhanced by a factor of 4-7 compared to conventional soft x-ray photoelectron spectroscopy at about 1000 keV. HXPS probes, on average, as far as 76 Å into the Fe <sub>x</sub>Si<sub>1-x</sub> samples. Via core-level spectra, it is found in the amorphous alloy that, in spite of the disordered structure that could lead to a broad distribution of chemical environments, the Si environment is mostly unique. Valence-band spectra reveal a clear distinction between the contributions of the two inequivalent Fe sites of the most highly ordered (x = 0.72, D0<sub>3</sub>) epitaxial sample. The valence-band spectra are compared to results of fully relativistic coherent potential approximation calculations performed in the framework of the one-step model of photoemission, which reveal details of the atomic-orbital makeup of various features, and generally exhibit good agreement with experiment.</p>