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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Felton, Solveig
Queen's University Belfast
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (14/14 displayed)
- 2022Thermal and magnetic field switching in a two-step hysteretic MnIII spin crossover compound coupled to symmetry breakingscitations
- 2022Thermal and Magnetic Field Switching in a Two‐Step Hysteretic Mn<sup>III</sup> Spin Crossover Compound Coupled to Symmetry Breakingscitations
- 2022Thermal and Magnetic Field Switching in a Two‐Step Hysteretic Mn(III) Spin Crossover Compound Coupled to Symmetry Breakingscitations
- 2022Thermal and magnetic field switching in a two-step hysteretic Mn III spin crossover compound coupled to symmetry breakingscitations
- 2021Percolation in metal-insulator composites of randomly packed spherocylindrical nanoparticlescitations
- 2019Controlling Ferromagnetic Ground States and Solitons in Thin Films and Nanowires Built from Iron Phthalocyanine Chainscitations
- 2016Evaluation of La1−xSrxMnO3 (0 ≤ x < 0.4) synthesised via a modified sol–gel method as mediators for magnetic fluid hyperthermiacitations
- 2006Simulations of magnetic microstructure in thin film elements used for programmable motion of magnetic particlescitations
- 2006Chemical tuning of the interlayer magnetic coupling in TlCo2Se2-xSxcitations
- 2005Cycloidal magnetic order in the compound IrMnSicitations
- 2005Magnetic short-range order in the new ternary phase Mn8Pd15Si7citations
- 2004Magnetic and electronic structure of TICo2S2citations
- 2004Crystal and magnetic structure of Mn3IrSicitations
- 2001Fragility of the spin-glass-like collective state to a magnetic field in an interacting Fe-C nanoparticle systemcitations
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article
Cycloidal magnetic order in the compound IrMnSi
Abstract
A new compound, IrMnSi, has been synthesized, and its crystal structure and magnetic properties have been investigated by means of neutron powder diffraction, magnetization measurements, and first-principles theory. The crystal structure is found to be of the TiNiSi type (ordered Co2P, space group Pnma). The Mn-projected electronic states are situated at the Fermi level, giving rise to metallic binding, whereas a certain degree of covalent character is observed for the chemical bond between the It and Si atoms. A cycloidal, i.e., noncollinear, magnetic structure was observed below 460 K, with the propagation vector q=[0,0,0.4530(5)] at 10 K. The magnetism is dominated by large moments on the Mn sites, 3.8 mu(B)/atom from neutron diffraction. First-principles theory reproduces the propagation vector of the experimental magnetic structure as well as the angles between the Mn moments. The calculations further result in a magnetic moment of 3.21 mu(B) for the Mn atoms, whereas the Ir and Si moments are negligible, in agreement with observations. A calculation that more directly incorporates electron-electron interactions improves the agreement between the theoretical and experimental magnetic moments. A band mechanism is suggested to explain the observed magnetic order.