| People | Locations | Statistics |
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| Naji, M. |
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| Motta, Antonella |
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| Aletan, Dirar |
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| Mohamed, Tarek |
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| Ertürk, Emre |
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| Taccardi, Nicola |
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| Kononenko, Denys |
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| Petrov, R. H. | Madrid |
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| Alshaaer, Mazen | Brussels |
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| Bih, L. |
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| Casati, R. |
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| Muller, Hermance |
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| Kočí, Jan | Prague |
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| Šuljagić, Marija |
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| Kalteremidou, Kalliopi-Artemi | Brussels |
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| Azam, Siraj |
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| Ospanova, Alyiya |
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| Blanpain, Bart |
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| Ali, M. A. |
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| Popa, V. |
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| Rančić, M. |
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| Ollier, Nadège |
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| Azevedo, Nuno Monteiro |
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| Landes, Michael |
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| Rignanese, Gian-Marco |
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Coak, Matthew John
University of Birmingham
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (6/6 displayed)
- 2024Magnetotransport of Sm2Ir2O7 across the pressure-induced quantum-critical phase boundarycitations
- 2023Asymmetric phase diagram and dimensional crossover in a system of spin-1/2 dimers under applied hydrostatic pressurecitations
- 2022Pressure-induced shift of effective Ce valence, Fermi energy and phase boundaries in CeOs4Sb12citations
- 2021Pressure-induced large increase of Curie temperature of the van der Waals ferromagnet VI3citations
- 2021Emergent magnetic phases in pressure-tuned van der Waals antiferromagnet FePS3citations
- 2015Low Temperature Resistivity of the Rare Earth Diborides (Er, Ho, Tm)B$_2$
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article
Asymmetric phase diagram and dimensional crossover in a system of spin-1/2 dimers under applied hydrostatic pressure
Abstract
We present the magnetic and structural properties of [Cu (pyrazine)<sub>0.5</sub> (glycine)] ClO<sub>4 </sub>under applied pressure. As previously reported, at ambient pressure this material consists of quasi-two-dimensional layers of weakly coupled antiferromagnetic dimers which undergo Bose-Einstein condensation of triplet excitations between two magnetic field-induced quantum critical points (QCPs). The molecular building blocks from which the compound is constructed give rise to exchange strengths that are considerably lower than those found in other <br/>S =1/2 dimer materials, which allows us to determine the pressure evolution of the entire field-temperature magnetic phase diagram using radio-frequency magnetometry. We find that a distinct phase emerges above the upper field-induced transition at elevated pressures and also show that an additional QCP is induced at zero field at a critical pressure of p<sub>c</sub> =15.7(5) kbar. Pressure-dependent single-crystal x-ray diffraction and density functional theory calculations indicate that this QCP arises primarily from a dimensional crossover driven by an increase in the interdimer interactions between the planes. While the effect of quantum fluctuations on the lower field-induced transition is enhanced with applied pressure, quantum Monte Carlo calculations suggest that this alone cannot explain an unconventional asymmetry that develops in the phase diagram.