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Rafferty, Niamh
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article
The Effects of Amino Acid Functionalisation on the Optoelectronic Properties and Self-Assembly of Perylene Bisimides
Abstract
<jats:title>Abstract</jats:title><jats:p>Here we report on ten water-soluble perylene bisimides (PBIs) that are functionalised with the amino acids L-alanine, L-aspartic acid, L-glutamic acid, L-phenylalanine, L-histidine, L-leucine, L-methionine, L-valine, L-tryptophan, and L-tyrosine. Reduction potentials, absoprtion and emission spectra, molar absorptivity, quantum yield, and rheology are obtained and the data interpreted for each species in aqueous solution or hydrogels in order to provide a comprehensive understanding of the subtle effects of amino acid functionalisation on the optoelectronic and supramolecular properties. The potential application of these PBIs in various organic electronic devices is assessed to demonstrate the importance of utilizing environmentally friendly solvents in material synthesis and processing and device manufacture.&#xD;</jats:p>