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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Lippert, Thomas
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (37/37 displayed)
- 2024Correlation of structural and magnetic properties of RFeO3 (R= Dy,Lu)citations
- 2024Correlation of structural and magnetic properties of RFeO$_3$ (R= Dy, Lu)
- 2024Thermally Stable Capacitive Energy-Density and Colossal Electrocaloric and Pyroelectric Effects of Sm-Doped Pb(Mg 1/3 Nb 2/3 )O 3 –PbTiO 3 Thin Filmscitations
- 2023Momentum-resolved electronic structure of LaTiO2N photocatalysts by resonant Soft-X-ray ARPEScitations
- 2023PLD plasma plume analysis: a summary of the PSI contributioncitations
- 2022Large imprint in epitaxial 0.67Pb(Mg<sub>1/3</sub>Nb<sub>2/3</sub>)O<sub>3</sub>-0.33PbTiO<sub>3</sub> thin films for piezoelectric energy harvesting applicationscitations
- 2021Heteroepitaxial Hexagonal (00.1) CuFeO2 Thin Film Grown on Cubic (001) SrTiO3 Substrate Through Translational and Rotational Domain Matchingcitations
- 2020Thickness-dependent microstructural properties of heteroepitaxial (00.1) CuFeO2 thin films on (00.1) sapphire by pulsed laser depositioncitations
- 2019Zigzag or spiral-shaped nanostructures improve mechanical stability in yttria-stabilized zirconia membranes for micro-energy conversion devicescitations
- 2017Anisotropic Proton and Oxygen Ion Conductivity in Epitaxial Ba2In2O5 Thin Filmscitations
- 2017Anisotropic Proton and Oxygen Ion Conductivity in Epitaxial Ba 2 In 2 O 5 Thin Filmscitations
- 2016TiN-buffered substrates for photoelectrochemical measurements of oxynitride thin filmscitations
- 2016The importance of pressure and mass ratios when depositing multi-element oxide thin films by pulsed laser depositioncitations
- 2015Probing the bulk ionic conductivity by thin film hetero-epitaxial engineeringcitations
- 2015Dense zig-zag microstructures in YSZ thin films by pulsed laser depositioncitations
- 2014A study of photothermal laser ablation of various polymers on microsecond time scalescitations
- 2014Laser deposition and direct-writing of thermoelectric misfit cobaltite thin filmscitations
- 2013On Proton Conductivity in Porous and Dense Yttria Stabilized Zirconia at Low Temperaturecitations
- 2013SIMS of thin films grown by pulsed laser deposition on isotopically labeled substratescitations
- 2012Strain and lattice distortion in (1 1 0)-epitaxial orthorhombic TbMnO3 multiferroic thin films grown by pulsed laser depositioncitations
- 2011Crystallization and grain growth characteristics of yttria-stabilized zirconia thin films grown by pulsed laser depositioncitations
- 2011Laser-induced ablation dynamics and flight of thin polymer filmscitations
- 2010The effects of switching time and SrTiO 3-x N y nanostructures on the operation of Al/SrTiO 3-x N y /Al memristorscitations
- 2010Laser-induced forward transfer of organic LED building blocks studied by time-resolved shadowgraphycitations
- 2010Laser ablation characteristics of yttria-doped zirconia in the nanosecond and femtosecond regimescitations
- 2010Pulsed laser deposition of gadolinia doped ceria layers at moderate temperature – a seeding approach
- 2009Micro-patterning for polymer electrolyte fuel cells: Single pulse laser ablation of aluminium films from glassy carboncitations
- 2009Characterization and properties of microwave plasma-treated SrTiO 3citations
- 2009Optical properties of nitrogen-substituted strontium titanate thin films prepared by pulsed laser depositioncitations
- 2008Aryltriazene photopolymer thin films as sacrificial release layers for laser-assisted forward transfer systems: study of photoablative decomposition and transfer behaviorcitations
- 2008Micro-patterning for polymer electrolyte fuel cells: single pulse laser ablation of aluminum films from glassy carboncitations
- 2007One-step preparation of N-doped strontium titanate films by pulsed laser depositioncitations
- 2007Fabrication of organic light-emitting diode pixels by laser-assisted forward transfercitations
- 2007Laser-produced plasma ion characteristics in laser ablation of lithium manganatecitations
- 2007The effect of the fluence on the properties of La–Ca–Mn–O thin films prepared by pulsed laser depositioncitations
- 2006Structure and composition of nanoscopic domains in functional perovskite-type materialscitations
- 2006Structural characterization and magnetoresistance of manganates thin films and Fe-doped manganates thin filmscitations
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article
Large imprint in epitaxial 0.67Pb(Mg<sub>1/3</sub>Nb<sub>2/3</sub>)O<sub>3</sub>-0.33PbTiO<sub>3</sub> thin films for piezoelectric energy harvesting applications
Abstract
<jats:p> Tuning and stabilizing a large imprint in epitaxial relaxor ferroelectric thin films is one of the key factors for designing micro-electromechanical devices with an enhanced figure of merit (FOM). In this work, epitaxial 500 nm-thick 0.67Pb(Mg<jats:sub>1/3</jats:sub>Nb<jats:sub>2/3</jats:sub>)O<jats:sub>3</jats:sub>–0.33PbTiO<jats:sub>3</jats:sub> (PMN–33PT) films, free from secondary phases and with extremely low rocking curves (FWHM < 0.05°), are grown on ScSmO<jats:sub>3</jats:sub> (SSO) and DyScO<jats:sub>3</jats:sub> (DSO) substrates buffered with SrRuO<jats:sub>3</jats:sub> (SRO). The PMN–33PT is observed to grow coherently on SSO substrates (lattice mismatch of −0.7%), which is c-axis oriented and exhibits large tetragonality compared to bulk PMN–33PT, while on DSO substrates (lattice mismatch of −1.9%), the PMN–33PT film is almost completely relaxed and shows reduced tetragonality. Due to the compressive epitaxial strain, the fully strained PMN–33PT film displays typical ferroelectric P–E hysteresis loops, while the relaxed sample shows relaxor-like P–E loops. Samples present large negative imprints of about −88.50 and −49.25 kV/cm for PMN–33PT/SRO/SSO and PMN–33PT/SRO/DSO, respectively, which is more than threefold higher than the coercive field. The imprint is induced by the alignment of defect dipoles with the polarization and is tuned by the epitaxial strain. It permits the stabilization of a robust positive polarization state (P<jats:sub>r</jats:sub> ∼ 20 μC/cm<jats:sup>2</jats:sup>) and low dielectric permittivity (<700). In addition, the relaxed PMN–33PT film shows improved piezoelectric properties, with a 33% enhancement in d<jats:sub>33,eff</jats:sub> relative to the fully strained sample. The obtained low dielectric permittivity and the high piezoelectric coefficients at zero electric field in the studied PMN–33PT films hold great promise to maximize the FOM toward applications in piezoelectric devices. </jats:p>