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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Loi, Maria Antonietta
University of Groningen
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (73/73 displayed)
- 2024Crystal Orientation, Strain, and Microstrain of Perovskite Films in a Complex Compositional Parameter Spacecitations
- 2024Understanding the Surface Chemistry of SnO 2 Nanoparticles for High Performance and Stable Organic Solar Cellscitations
- 2024Cation Influence on Hot-Carrier Relaxation in Tin Triiodide Perovskite Thin Filmscitations
- 2024Quasi-2D Lead–Tin Perovskite Memory Devices Fabricated by Blade Coatingcitations
- 2024PbI2 Passivation of Three Dimensional PbS Quantum Dot Superlattices Toward Optoelectronic Metamaterialscitations
- 2024Understanding the Surface Chemistry of SnO2 Nanoparticles for High Performance and Stable Organic Solar Cellscitations
- 2024Metal-Solvent Complex Formation at the Surface of InP Colloidal Quantum Dotscitations
- 2023Lead Sulfide Quantum Dots for Synaptic Transistors:Modulating the Learning Timescale with Ligandscitations
- 2023The Origin of Broad Emission in ⟨100⟩ Two-Dimensional Perovskites: Extrinsic vs Intrinsic Processes.
- 2023Unraveling the Broadband Emission in Mixed Tin-Lead Layered Perovskitescitations
- 2023Unraveling the Broadband Emission in Mixed Tin-Lead Layered Perovskitescitations
- 2023Impact of two diammonium cations on the structure and photophysics of layered Sn-based perovskitescitations
- 2023A carbazole-based self-assembled monolayer as the hole transport layer for efficient and stable Cs 0.25 FA 0.75 Sn 0.5 Pb 0.5 I 3 solar cellscitations
- 2023Introduction to halide perovskite optoelectronicscitations
- 2023Lead Sulfide Quantum Dots for Synaptic Transistorscitations
- 2023Tuning the energy transfer in Ruddlesden-Popper perovskites phases through isopropylammonium addition - towards efficient blue emitterscitations
- 2023Tuning the energy transfer in Ruddlesden–Popper perovskites phases through isopropylammonium addition – towards efficient blue emitterscitations
- 2023Disentangling Dual Emission Dynamics in Lead Bromide Perovskitecitations
- 2023Disentangling Dual Emission Dynamics in Lead Bromide Perovskitecitations
- 2023Addition of Ammonium Thiocyanate Alters the Microstructure and Energetic Landscape of 2D/3D Perovskite Films
- 2022Direct measurement of radiative decay rates in metal halide perovskites†citations
- 2022The Origin of Broad Emission in â ¨100»Two-Dimensional Perovskites: Extrinsic vs Intrinsic Processes
- 2022Taking a closer look - how the microstructure of Dion-Jacobson perovskites governs their photophysics
- 2022Taking a closer look - how the microstructure of Dion-Jacobson perovskites governs their photophysicscitations
- 2021Photophysics of Two-Dimensional Perovskites—Learning from Metal Halide Substitutioncitations
- 2021Photophysics of Two-Dimensional Perovskites—Learning from Metal Halide Substitution
- 2021Brightening of dark excitons in 2D perovskitescitations
- 2021Crystallization driven boost in fill factor and stability in additive-free organic solar cellscitations
- 2021Crystallization driven boost in fill factor and stability in additive-free organic solar cellscitations
- 2021Molecular Doping Directed by a Neutral Radicalcitations
- 2021Molecular Doping Directed by a Neutral Radicalcitations
- 2021Scalable, Template Driven Formation of Highly Crystalline Lead-Tin Halide Perovskite Filmscitations
- 2021Scalable, Template Driven Formation of Highly Crystalline Lead-Tin Halide Perovskite Filmscitations
- 2020Negative Thermal Quenching in FASnI3 Perovskite Single Crystals and Thin Filmscitations
- 2020Broad Tunability of Carrier Effective Masses in Two-Dimensional Halide Perovskitescitations
- 2020Unraveling the Microstructure of Layered Metal Halide Perovskite Filmscitations
- 2020Extrinsic nature of the broad photoluminescence in lead iodide-based Ruddlesden-Popper perovskitescitations
- 2020Stable cesium formamidinium lead halide perovskites: a comparison of photophysics and phase purity in thin films and single crystalscitations
- 2019Stable Cesium Formamidinium Lead Halide Perovskitescitations
- 2019Mechanism of surface passivation of methylammonium lead tribromide single crystals by benzylaminecitations
- 2019Constructing the Electronic Structure of CH3NH3PbI3 and CH3NH3PbBr3 Perovskite Thin Films from Single-Crystal Band Structure Measurementscitations
- 2019Enhancing the crystallinity and perfecting the orientation of formamidinium tin iodide for highly efficient Sn-based perovskite solar cellscitations
- 2019Scalable fabrication of high-quality crystalline and stable FAPbI(3) thin films by combining doctor-blade coating and the cation exchange reactioncitations
- 2019Scalable fabrication of high-quality crystalline and stable FAPbI(3) thin films by combining doctor-blade coating and the cation exchange reactioncitations
- 2019Favorable Mixing Thermodynamics in Ternary Polymer Blends for Realizing High Efficiency Plastic Solar Cellscitations
- 2019Photophysical and electronic properties of bismuth-perovskite shelled lead sulfide quantum dotscitations
- 2019The Impact of Stoichiometry on the Photophysical Properties of Ruddlesden-Popper Perovskitescitations
- 2019Stable Cesium Formamidinium Lead Halide Perovskites:A Comparison of Photophysics and Phase Purity in Thin Films and Single Crystalscitations
- 2019Effects of strontium doping on the morphological, structural, and photophysical properties of FASnI(3) perovskite thin filmscitations
- 2018Perovskite Excitonics:Primary Exciton Creation and Crossover from Free Carriers to a Secondary Exciton Phasecitations
- 2018Micropatterned 2D Hybrid Perovskite Thin Films with Enhanced Photoluminescence Lifetimescitations
- 2018Interfacial Morphology Addresses Performance of Perovskite Solar Cells Based on Composite Hole Transporting Materials of Functionalized Reduced Graphene Oxide and P3HTcitations
- 2018Lead-Chalcogenide Colloidal-Quantum-Dot Solids:Novel Assembly Methods, Electronic Structure Control, and Application Prospectscitations
- 2018Perovskite Excitonics: Primary Exciton Creation and Crossover from Free Carriers to a Secondary Exciton Phasecitations
- 2017Stoichiometric control of the density of states in PbS colloidal quantum dot solidscitations
- 2017Broadly tunable metal halide perovskites for solid-state light-emission applicationscitations
- 2016Confinement Effects in Low-Dimensional Lead Iodide Perovskite Hybridscitations
- 2016Theoretical and experimental insights into hybrid perovskites for optoelectronic applications
- 2015Polyazines and Polyazomethines with Didodecylthiophene Units for Selective Dispersion of Semiconducting Single-Walled Carbon Nanotubescitations
- 2015Photophysics of Organic-Inorganic Hybrid Lead Iodide Perovskite Single Crystalscitations
- 2015Photophysics of Organic-Inorganic Hybrid Lead Iodide Perovskite Single Crystalscitations
- 2015Inside Front Cover: Hybrid Perovskites: Photophysics of Organic–Inorganic Hybrid Lead Iodide Perovskite Single Crystals (Adv. Funct. Mater. 16/2015)citations
- 2015High Mobility and Low Density of Trap States in Dual-Solid-Gated PbS Nanocrystal Field-Effect Transistorscitations
- 2014Determination of the Electronic Energy Levels of Colloidal Nanocrystals using Field-Effect Transistors and Ab-Initio Calculationscitations
- 2013Low Driving Voltage and High Mobility Ambipolar Field-Effect Transistors with PbS Colloidal Nanocrystalscitations
- 2013Hybrid solar cells:Perovskites under the Suncitations
- 2012Charge transfer state in highly efficient polymer-fullerene bulk heterojunction solar cellscitations
- 2011Sensitive triplet exciton detection in polyfluorene using Pd-coordinated porphyrincitations
- 2011Infrared Emitting and Photoconducting Colloidal Silver Chalcogenide Nanocrystal Quantum Dots from a Silylamide-Promoted Synthesiscitations
- 2009Solution-Processable Near-IR Photodetectors Based on Electron Transfer from PbS Nanocrystals to Fullerene Derivativescitations
- 2009Exciton Quenching Close to Polymer-Vacuum Interface of Spin-Coated Films of Poly(p-phenylenevinylene) Derivativecitations
- 2008Quasi-seeded growth of ligand-tailored PbSe nanocrystals through cation-exchange-mediated nucleationcitations
- 2005Correlation Between Morphology and Field-Effect-Transistor Mobility in Tetracene Thin Filmscitations
Places of action
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article
Photophysical and electronic properties of bismuth-perovskite shelled lead sulfide quantum dots
Abstract
Metal halide perovskite shelled quantum dot solids have recently emerged as an interesting class of solution-processable materials that possess the desirable electronic properties of both quantum dots and perovskites. Recent reports have shown that lead sulfide quantum dots (PbS QDs) with perovskite ligand-shells can be successfully utilized in (opto)electronic devices such as solar cells, photoconductors, and field-effect transistors (FETs), a development attributed to the compatibility of lattice parameters between PbS and certain metal halide perovskites that results in the growth of the perovskite shell on the PbS QDs. Of several possible perovskite combinations used with PbS QDs, bismuth-based variants have been shown to have the lowest lattice mismatch and to display excellent performance in photoconductors. However, they also display photoluminescence (PL), which is highly sensitive to surface defects. In this work, we present an investigation of the transport and optical properties of two types of bismuth-based perovskite (MA(3)BiI(6) and MA(3)Bi(2)I(9)) shelled PbS QDs. Our photophysical study using temperature-dependent PL spectroscopy between 5 and 290 K indicates that the PL efficiency of the reference oleic acid (OA) capped samples is much higher than that of the Bi-shelled ones, which suffer from traps, most likely formed at their surfaces during the phase-transfer ligand exchange process. Nevertheless, the results from electrical measurements on FETs show the successful removal of the native-OA ligands, displaying electron dominated transport with modest mobilities of around 10(-3) cm(2) [V s](-1) - comparable to the reported values for epitaxial Pb-based shelled samples. These findings advance our understanding of perovskite shelled QD-solids and point to the utility of these Bi-based variants as contenders for photovoltaic and other optoelectronic applications. Published under license by AIP Publishing.