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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Bibes, Manuel
French National Centre for Scientific Research
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (25/25 displayed)
- 2024Origin of the Surface Magnetic Dead Layer in Rare‐Earth Titanates
- 2024Ferroelectric spin orbit devices for ultralow power computing
- 2024Unraveling P‐Type and N‐Type Interfaces in Superconducting Infinite‐Layer Nickelate Thin Filmscitations
- 2024Toward Reliable Synthesis of Superconducting Infinite Layer Nickelate Thin Films by Topochemical Reductioncitations
- 2024Toward Reliable Synthesis of Superconducting Infinite Layer Nickelate Thin Films by Topochemical Reductioncitations
- 2023Epitaxial growth of the candidate ferroelectric Rashba material SrBiO<sub>3</sub> by pulsed laser deposition
- 2022Strain tuning of Néel temperature in YCrO 3 epitaxial thin filmscitations
- 2021Depth profile reconstruction of YCrO3 / CaMnO3 superlattices by near total reflection HAXPEScitations
- 2021Spin–Charge Interconversion in KTaO 3 2D Electron Gasescitations
- 2021Surface and bulk ferroelectric phase transition in super-tetragonal BiFeO 3 thin filmscitations
- 2021Spin–Charge Interconversion in KTaO3 2D Electron Gasescitations
- 2021Room-temperature ferroelectric switching of spin-to-charge conversion in GeTecitations
- 2021Room-temperature ferroelectric switching of spin-to-charge conversion in germanium telluridecitations
- 2020Ultrafast spin-currents and charge conversion at 3d-5d interfaces probed by time-domain terahertz spectroscopycitations
- 2020Switchable two-dimensional electron gas based on ferroelectric Ca:SrTiO 3citations
- 2020Interfacial Strain Gradients Control Nanoscale Domain Morphology in Epitaxial BiFeO 3 Multiferroic Filmscitations
- 2020Interfacial Strain Gradients Control Nanoscale Domain Morphology in Epitaxial BiFeO3 Multiferroic Filmscitations
- 2019Switching on superferromagnetismcitations
- 2019Imaging and Harnessing Percolation at the Metal–Insulator Transition of NdNiO 3 Nanogapscitations
- 2019Electrically Switchable and Tunable Rashba-Type Spin Splitting in Covalent Perovskite Oxidescitations
- 2019A magnetic phase diagram for nanoscale epitaxial BiFeO3 filmscitations
- 2019A magnetic phase diagram for nanoscale epitaxial BiFeO 3 filmscitations
- 2018Oxide spin-orbitronics: New routes towards low-power electrical control of magnetization in oxide heterostructurescitations
- 2016Large elasto-optic effect and reversible electrochromism in multiferroic BiFeO3citations
- 2014Linear electro-optic effect in multiferroic BiFeO3 thin filmscitations
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article
A magnetic phase diagram for nanoscale epitaxial BiFeO3 films
Abstract
<jats:p>BiFeO3 thin films have attracted considerable attention by virtue of their potential application in low-energy spintronic and magnonic devices. BiFeO3 possesses an intricate magnetic structure, characterized by a spin cycloid with period ∼62 nm that governs the functional magnonic response, and which can be modulated or even destroyed by strain, magnetic and electric fields, or chemical doping. The literature on (110)-oriented BiFeO3 films is not explicit in defining the conditions under which this cycloid persists, as its presence depends on synthesis method and thin-film boundary conditions, especially in the sub-100 nm thickness regime. This report aims to end “trial and error” approaches in determining the conditions under which this cycloid and its associated functional magnonic response exist. We show that in specific crystallographic orientations of epitaxial BiFeO3, an unexplored strain parameter—the distortion in the ab plane of the monoclinic unit cell—significantly influences the spin structure. Combining Mössbauer spectroscopy and low-energy Raman spectroscopy with first-principles-based effective Hamiltonian calculations, we show that both average strain and this distortion destroy the cycloid. For films grown on (110)-oriented SrTiO3 substrates, if the BiFeO3 lattice parameters a and b differ by more than about 1.2%, the cycloid is destabilized, resulting in a pseudocollinear magnetic order ground state. We are thereby able to construct a phase diagram of the spin structure for nanoscale epitaxial BiFeO3 films, which aims to resolve long-standing literature inconsistencies and provide powerful guidelines for the design of future magnonic and spintronic devices.</jats:p>