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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Borgatti, F.
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (16/16 displayed)
- 2021Identification of hidden orbital contributions in the La_{0.65} Sr_{0.35} MnO_{3} valence band
- 2021Identification of hidden orbital contributions in the La$_{0.65}$Sr$_{0.35}$MnO$_3$ valence bandcitations
- 2021Identification of hidden orbital contributions in the La0.65Sr0.35MnO3 valence bandcitations
- 2020Direct insight into the band structure of SrNbO3citations
- 2018Charge-transfer in B-site-depleted NdGaO3/SrTiO3 heterostructurescitations
- 2017Quantifying the critical thickness of electron hybridization in spintronics materialscitations
- 2017Quantifying the critical thickness of electron hybridization in spintronics materialscitations
- 2016Observation of Distinct Bulk and Surface Chemical Environments in a Topological Insulator under Magnetic dopingcitations
- 2016Role and optimization of the active oxide layer in TiO2-based RRAMcitations
- 2014Synthesis of Bismuth-Based Materials by Electrodeposition
- 2014A combined ion scattering, photoemission, and DFT investigation on the termination layer of a La0.7Sr0.3MnO3 spin injecting electrodecitations
- 2013Conditions for the growth of smooth La0.7Sr0.3MnO3 thin films by pulsed electron ablationcitations
- 2012Surface X-ray diffraction analysis of Fe nanostructured films grown on c(2×2)-N/Cu(100)citations
- 2008Room-temperature spintronic effects in Alq3-based hybrid devicescitations
- 2002Anisotropy in c-oriented MgB2 thin films grown by pulsed laser depositioncitations
- 2001Growth of c-oriented MgB2 thin films by pulsed laser deposition: structural characterization and electronic anisotropycitations
Places of action
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article
Charge-transfer in B-site-depleted NdGaO3/SrTiO3 heterostructures
Abstract
<p>Cation stoichiometry has been identified as a major key in establishing 2-dimensional electron gases (2DEGs) in oxide heterostructures. Here, we discuss a 2DEG formation scenario in B-site deficient perovskite/perovskite heterostructures, which previously were predicted to show insulating behavior. We elaborate an ionic picture based on oxygen-vacancy-buffered B-site vacancy defects in the polar oxide layer that yields a continuous transition from 2DEG formation to less conducting interfaces to insulating interfaces with increasing B-site deficiency. Experimentally, a corresponding modulation of charge transfer across NdGaO<sub>3</sub>/SrTiO<sub>3</sub> interfaces is inferred using hard x-ray photoelectron spectroscopy analysis and transport experiments. With increasing B-site deficiency, we observe a decrease of the interfacial Ti<sup>3+</sup> core level contribution, indicating a reduced charge transfer at the interface. This result is corroborated by temperature-dependent transport measurements, revealing increased low temperature resistance, with a dominant influence of a reduced electron density in the Ga-depleted sample. We consider a redistribution of oxygen vacancies in the B-site deficient polar oxide layer to explain the alleviated interface reconstruction, adding a new perspective on potential built-up in polar-oxide thin films.</p>