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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Hoogland, Sjoerd
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Topics
Publications (9/9 displayed)
- 2023Sequential Co‐Passivation in InAs Colloidal Quantum Dot Solids Enables Efficient Near‐Infrared Photodetectorscitations
- 2022Engineering Electro‐Optic BaTiO<sub>3</sub> Nanocrystals via Efficient Dopingcitations
- 2019Nanostructured Back Reflectors for Efficient Colloidal Quantum-Dot Infrared Optoelectronics
- 2019Lattice anchoring stabilizes solution-processed semiconductorscitations
- 2017Hybrid tandem quantum dot/organic photovoltaic cells with complementary near infrared absorptioncitations
- 2016Ligand-Stabilized Reduced-Dimensionality Perovskitescitations
- 2016Amine-Free Synthesis of Cesium Lead Halide Perovskite Quantum Dots for Efficient Light-Emitting Diodescitations
- 2015Planar-integrated single-crystalline perovskite photodetectorscitations
- 2015Two-Photon Absorption in Organometallic Bromide Perovskitescitations
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article
Hybrid tandem quantum dot/organic photovoltaic cells with complementary near infrared absorption
Abstract
Monolithically integrated hybrid tandem solar cells that effectively combine solution-processed colloidal quantum dot (CQD) and organic bulk heterojunction subcells to achieve tandem performance that surpasses the individual subcell efficiencies have not been demonstrated to date. In this work, we demonstrate hybrid tandem cells with a low bandgap PbS CQD subcell harvesting the visible and near-infrared photons and a polymer:fullerene—poly (diketopyrrolopyrrole-terthiophene) (PDPP3T):[6,6]-phenyl-C60-butyric acid methyl ester (PC61BM)—top cell absorbing effectively the red and near-infrared photons of the solar spectrum in a complementary fashion. The two subcells are connected in series via an interconnecting layer (ICL) composed of a metal oxide layer, a conjugated polyelectrolyte, and an ultrathin layer of Au. The ultrathin layer of Au forms nano-islands in the ICL, reducing the series resistance, increasing the shunt resistance, and enhancing the device fill-factor. The hybrid tandems reach a power conversion efficiency (PCE) of 7.9%, significantly higher than the PCE of the corresponding individual single cells, representing one of the highest efficiencies reported to date for hybrid tandem solar cells based on CQD and polymer subcells.