Materials Map

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The Materials Map is an open tool for improving networking and interdisciplinary exchange within materials research. It enables cross-database search for cooperation and network partners and discovering of the research landscape.

The dashboard provides detailed information about the selected scientist, e.g. publications. The dashboard can be filtered and shows the relationship to co-authors in different diagrams. In addition, a link is provided to find contact information.

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The Materials Map is still under development. In its current state, it is only based on one single data source and, thus, incomplete and contains duplicates. We are working on incorporating new open data sources like ORCID to improve the quality and the timeliness of our data. We will update Materials Map as soon as possible and kindly ask for your patience.

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Publications (1/1 displayed)

  • 2023Limits to the strain engineering of layered square-planar nickelate thin films23citations

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Goodge, Berit
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Paik, Hanjong
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Mason, Jarad
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2023

Co-Authors (by relevance)

  • Goodge, Berit
  • Paik, Hanjong
  • Mason, Jarad
  • Kourkoutis, Lena F.
  • Baggari, Ismail El
  • Botana, Antia S.
  • Ferenc Segedin, Dan
  • Ndiaye, Alpha
  • Brooks, Charles M.
  • Doyle, Spencer
  • Taylor, Nicole K.
  • Mundy, Julia
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article

Limits to the strain engineering of layered square-planar nickelate thin films

  • Goodge, Berit
  • Paik, Hanjong
  • Mason, Jarad
  • Kourkoutis, Lena F.
  • Baggari, Ismail El
  • Botana, Antia S.
  • Ferenc Segedin, Dan
  • Ndiaye, Alpha
  • Brooks, Charles M.
  • Doyle, Spencer
  • Taylor, Nicole K.
  • Mundy, Julia
  • Labollita, Harrison
Abstract

<jats:title>Abstract</jats:title><jats:p>The layered square-planar nickelates, Nd<jats:sub><jats:italic>n</jats:italic>+1</jats:sub>Ni<jats:sub><jats:italic>n</jats:italic></jats:sub>O<jats:sub>2<jats:italic>n</jats:italic>+2</jats:sub>, are an appealing system to tune the electronic properties of square-planar nickelates via dimensionality; indeed, superconductivity was recently observed in Nd<jats:sub>6</jats:sub>Ni<jats:sub>5</jats:sub>O<jats:sub>12</jats:sub> thin films. Here, we investigate the role of epitaxial strain in the competing requirements for the synthesis of the <jats:italic>n</jats:italic> = 3 Ruddlesden-Popper compound, Nd<jats:sub>4</jats:sub>Ni<jats:sub>3</jats:sub>O<jats:sub>10</jats:sub>, and subsequent reduction to the square-planar phase, Nd<jats:sub>4</jats:sub>Ni<jats:sub>3</jats:sub>O<jats:sub>8</jats:sub>. We synthesize our highest quality Nd<jats:sub>4</jats:sub>Ni<jats:sub>3</jats:sub>O<jats:sub>10</jats:sub> films under compressive strain on LaAlO<jats:sub>3</jats:sub> (001), while Nd<jats:sub>4</jats:sub>Ni<jats:sub>3</jats:sub>O<jats:sub>10</jats:sub> on NdGaO<jats:sub>3</jats:sub> (110) exhibits tensile strain-induced rock salt faults but retains bulk-like transport properties. A high density of extended defects forms in Nd<jats:sub>4</jats:sub>Ni<jats:sub>3</jats:sub>O<jats:sub>10</jats:sub> on SrTiO<jats:sub>3</jats:sub> (001). Films reduced on LaAlO<jats:sub>3</jats:sub> become insulating and form compressive strain-induced <jats:italic>c</jats:italic>-axis canting defects, while Nd<jats:sub>4</jats:sub>Ni<jats:sub>3</jats:sub>O<jats:sub>8</jats:sub> films on NdGaO<jats:sub>3</jats:sub> are metallic. This work provides a pathway to the synthesis of Nd<jats:sub><jats:italic>n</jats:italic>+1</jats:sub>Ni<jats:sub><jats:italic>n</jats:italic></jats:sub>O<jats:sub>2<jats:italic>n</jats:italic>+2</jats:sub> thin films and sets limits on the ability to strain engineer these compounds via epitaxy.</jats:p>

Topics
  • density
  • compound
  • phase
  • thin film
  • layered
  • defect
  • superconductivity
  • superconductivity