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| Azevedo, Nuno Monteiro |
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Iwashina, Katsuya
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article
Z-schematic water splitting into H2 and O2 using metal sulfide as a hydrogen-evolving photocatalyst and reduced graphene oxide as a solid-state electron mediator
Abstract
Z-schematic water splitting was successfully demonstrated using metal sulfide photocatalysts that were usually unsuitable for water splitting as single particulate photocatalysts due to photocorrosion. When metal sulfide photocatalysts with a p-type semiconductor character as a H<sub>2</sub>-evolving photocatalyst were combined with reduced graphene oxide-TiO<sub>2</sub> composite as an O<sub>2</sub>-evolving photocatalyst, water splitting into H<sub>2</sub> and O<sub>2</sub> in a stoichiometric amount proceeded. In this system, photogenerated electrons in the TiO<sub>2</sub> with an n-type semiconductor character transferred to the metal sulfide through a reduced graphene oxide to achieve water splitting. Moreover, this system was active for solar water splitting.