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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Aizpurua, Javier
Donostia International Physics Center
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (13/13 displayed)
- 2024Unified treatment of light emission by inelastic tunneling: Interaction of electrons and photons beyond the gapcitations
- 2024Footprints of atomic-scale features in plasmonic nanoparticles as revealed by electron energy loss spectroscopycitations
- 2023Probing optical anapoles with fast electron beamscitations
- 2022Probing the role of grain boundaries in single Cu nanoparticle oxidation by in situ plasmonic scatteringcitations
- 2022Probing the role of grain boundaries in single Cu nanoparticle oxidation by in situ plasmonic scatteringcitations
- 2022Probing the role of grain boundaries in single Cu nanoparticle oxidation by in situ plasmonic scatteringcitations
- 2020Probing the radiative electromagnetic local density of states in nanostructures with a scanning tunneling microscopecitations
- 2020Probing the radiative electromagnetic local density of states in nanostructures with a scanning tunneling microscopecitations
- 2020Probing the radiative electromagnetic local density of states in nanostructures with a scanning tunneling microscopecitations
- 2019Gold‐ and Silver‐Coated Barium Titanate Nanocomposites as Probes for Two‐Photon Multimodal Microspectroscopycitations
- 2018Vibrational electron energy loss spectroscopy in truncated dielectric slabscitations
- 2018Surface-enhanced molecular electron energy loss spectroscopycitations
- 2017Probing low-energy hyperbolic polaritons in van der Waals crystals with an electron microscope
Places of action
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article
Probing the radiative electromagnetic local density of states in nanostructures with a scanning tunneling microscope
Abstract
A novel technique for the investigation of the radiative contribution to the electromagnetic local density of states is presented. The inelastic tunneling current from a scanning tunneling microscope (STM) is used to locally and electrically excite the plasmonic modes of a triangular gold platelet. The radiative decay of these modes is detected through the transparent substrate in the far field. Emission spectra, which depend on the position of the STM excitation, as well as energy-filtered emission maps for particular spectral windows are acquired using this technique. The STM-nanosource spectroscopy and microscopy results are compared to those obtained from spatially resolved electron energy loss spectroscopy (EELS) maps on similar platelets. While EELS is known to be related to the total projected electromagnetic local density of states, the light emission from the STM-nanosource is shown here to select the radiative contribution. Full electromagnetic calculations are carried out to explain the experimental STM data, and provide valuable insight into the radiative nature of the different contributions of the breathing and edge plasmon modes of the nanoparticles. Our results introduce the STM-nanosource as a tool to investigate and engineer light emission at the nanoscale.