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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Zhang, Lei
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (14/14 displayed)
- 2023The Parkes Pulsar Timing Array third data releasecitations
- 2022A Coarse-Grained Molecular Model for Simulating Self-Healing of Bitumencitations
- 2022A Coarse-Grained Molecular Model for Simulating Self-Healing of Bitumencitations
- 2020Manipulating magnetoelectric energy landscape in multiferroicscitations
- 2020Manipulating magnetoelectric energy landscape in multiferroicscitations
- 2018Continuously Tuning Epitaxial Strains by Thermal Mismatchcitations
- 2018Self-Suspended Nanomesh Scaffold for Ultrafast Flexible Photodetectors Based on Organic Semiconducting Crystalscitations
- 2016Improving the Stability of Organic Semiconductors: Distortion Energy versus Aromaticity in Substituted Bistetracenecitations
- 2015Effect of cooling rate on microstructure and properties of microalloyed HSLA steel weld metalscitations
- 2012Criteria for improving the properties of ZnGeAs2 solar cellscitations
- 2007An efficient hybrid, nanostructured, epoxidation catalyst: titanium silsesquioxane-polystyrene copolymer supported on SBA-15
- 2007An efficient hybrid, nanostructured, epoxidation catalyst: titanium silsesquioxane-polystyrene copolymer supported on SBA-15citations
- 2007An efficient hybrid, nanostructured, epoxidation catalyst: titanium silsesquioxane-polystyrene copolymer supported on SBA-15citations
- 2004Sidewall functionalization of single-walled carbon nanotubes with hydroxyl group-terminated moietiescitations
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article
Continuously Tuning Epitaxial Strains by Thermal Mismatch
Abstract
Strain engineering of thin films is a conventionally employed approach to enhance material properties and to energetically prefer ground states that would otherwise not be attainable. Controlling strain states in perovskite oxide thin films is usually accomplished through coherent epitaxy by using lattice-mismatched substrates with similar crystal structures. However, the limited choice of suitable oxide substrates makes certain strain states experimentally inaccessible and a continuous tuning impossible. Here, we report a strategy to continuously tune epitaxial strains in perovskite films grown on Si(001) by utilizing the large difference of thermal expansion coefficients between the film and the substrate. By establishing an adsorption-controlled growth window for SrTiO<sub>3</sub> thin films on Si using hybrid molecular beam epitaxy, the magnitude of strain can be solely attributed to thermal expansion mismatch, which only depends on the difference between growth and room temperature. Second-harmonic generation measurements revealed that structure properties of SrTiO<sub>3</sub> films could be tuned by this method using films with different strain states. Our work provides a strategy to generate continuous strain states in oxide/semiconductor pseudomorphic buffer structures that could help achieve desired material functionalities.