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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Ulstrup, Søren
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (18/18 displayed)
- 2022Visualizing band structure hybridization and superlattice effects in twisted MoS<sub>2</sub>/WS<sub>2</sub> heterobilayerscitations
- 2020Visualizing Orbital Content of Electronic Bands in Anisotropic 2D Semiconducting ReSe 2citations
- 2020Visualizing Orbital Content of Electronic Bands in Anisotropic 2D Semiconducting ReSe2citations
- 2019Imaging microscopic electronic contrasts at the interface of single-layer WS 2 with oxide and boron nitride substratescitations
- 2019Transient hot electron dynamics in single-layer TaS2citations
- 2019Transient hot electron dynamics in single-layer TaS2citations
- 2019Transient hot electron dynamics in single-layer TaS 2citations
- 2019Transient hot electron dynamics in single-layer TaS 2citations
- 2019Tunable electronic structure in gallium chalcogenide van der Waals compoundscitations
- 2018Giant spin-splitting and gap renormalization driven by trions in single-layer WS2/h- BN heterostructurescitations
- 2017Spin and valley control of free carriers in single-layer WS2citations
- 2017Ultrafast band structure control of a two-dimensional heterostructurecitations
- 2017Spin and valley control of free carriers in single-layer WS 2citations
- 2016Ultrafast Band Structure Control of a Two-Dimensional Heterostructurecitations
- 2016Ultrafast band structure control of a two-dimensional heterostructurecitations
- 2015Electronic structure of epitaxial single-layer MoS2citations
- 2015Synthesis of Epitaxial Single-Layer MoS 2 on Au(111)citations
- 2015Synthesis of Epitaxial Single-Layer MoS2 on Au(111)citations
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article
Ultrafast Band Structure Control of a Two-Dimensional Heterostructure
Abstract
<p>The electronic structure of two-dimensional (2D) semiconductors can be significantly altered by screening effects, either from free charge carriers in the material or by environmental screening from the surrounding medium. The physical properties of 2D semiconductors placed in a heterostructure with other 2D materials are therefore governed by a complex interplay of both intra- and interlayer interactions. Here, using time- and angle-resolved photoemission, we are able to isolate both the layer-resolved band structure and, more importantly, the transient band structure evolution of a model 2D heterostructure formed of a single layer of MoS<sub>2</sub> on graphene. Our results reveal a pronounced renormalization of the quasiparticle gap of the MoS<sub>2</sub> layer. Following optical excitation, the band gap is reduced by up to ∼400 meV on femtosecond time scales due to a persistence of strong electronic interactions despite the environmental screening by the n-doped graphene. This points to a large degree of tunability of both the electronic structure and the electron dynamics for 2D semiconductors embedded in a van der Waals-bonded heterostructure.</p>