| People | Locations | Statistics |
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| Naji, M. |
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| Motta, Antonella |
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| Aletan, Dirar |
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| Mohamed, Tarek |
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| Ertürk, Emre |
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| Taccardi, Nicola |
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| Kononenko, Denys |
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| Petrov, R. H. | Madrid |
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| Alshaaer, Mazen | Brussels |
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| Bih, L. |
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| Casati, R. |
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| Muller, Hermance |
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| Kočí, Jan | Prague |
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| Šuljagić, Marija |
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| Kalteremidou, Kalliopi-Artemi | Brussels |
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| Azam, Siraj |
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| Ospanova, Alyiya |
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| Blanpain, Bart |
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| Ali, M. A. |
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| Popa, V. |
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| Rančić, M. |
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| Ollier, Nadège |
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| Azevedo, Nuno Monteiro |
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| Landes, Michael |
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| Rignanese, Gian-Marco |
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Rizzi, Gian Andrea
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (15/15 displayed)
- 2024Pt-decorated graphitic carbon nitride on carbon paper by x-ray photoelectron spectroscopycitations
- 2023Insights into the Photoelectrocatalytic Behavior of gCN-Based Anode Materials Supported on Ni Foamscitations
- 2023Fe2O3-graphitic carbon nitride nanocomposites analyzed by XPScitations
- 2018Density Functional Theory (DFT) and Experimental Evidences of Metal–Support Interaction in Platinum Nanoparticles Supported on Nitrogen- and Sulfur-Doped Mesoporous Carbons: Synthesis, Activity, and Stabilitycitations
- 2018Interfacial Morphology Addresses Performance of Perovskite Solar Cells Based on Composite Hole Transporting Materials of Functionalized Reduced Graphene Oxide and P3HTcitations
- 2018Probing the correlation between Pt-support interaction and oxygen reduction reaction activity in mesoporous carbon materials modified with Pt-N active sitescitations
- 2017Ag-Vanadates/GO Nanocomposites by Aerosol-Assisted Spray Pyrolysis: Preparation and Structural and Electrochemical Characterization of a Versatile Materialcitations
- 2016VO <sub>2</sub> /V <sub>2</sub> O <sub>5</sub> :Ag Nanostructures on a DVD as Photoelectrochemical Sensorscitations
- 2016Cu2O/TiO2 heterostructures on a DVD as easy&cheap photoelectrochemical sensorscitations
- 2015Comparison between the Oxygen Reduction Reaction Activity of Pd<sub>5</sub>Ce and Pt<sub>5</sub>Ce: The Importance of Crystal Structurecitations
- 2013Xylene sensing properties of aryl-bridged polysilsesquioxane thin films coupled to gold nanoparticlescitations
- 2005Epitaxial TiO2 nanoparticles on Pt(111): a structural study by photoelectron diffraction and scanning tunneling microscopycitations
- 2005Ultrathin TiO<i><sub>x</sub></i> Films on Pt(111): A LEED, XPS, and STM Investigationcitations
- 2003Growth of NiO ultrathin films on Pd(100) by post-oxidation of Ni films: the effect of pre-adsorbed oxygencitations
- 2000An X-ray photoelectron diffraction structural characterisation of epitaxial ultrathin RuO2/TiO2(110) films obtained by decomposition of Ru3(CO)12citations
Places of action
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article
Density Functional Theory (DFT) and Experimental Evidences of Metal–Support Interaction in Platinum Nanoparticles Supported on Nitrogen- and Sulfur-Doped Mesoporous Carbons: Synthesis, Activity, and Stability
Abstract
In this paper, we report a comprehensive investigation of Pt nanoparticles (NPs) deposition on nitrogen- and sulfur-doped or codoped mesoporous carbons (N-MC, S-MC, and N,S-MC) to develop active and durable oxygen reduction catalysts for fuel cells. N-MC, S-MC, and N,S-MC were prepared by employing mesoporous silica as hard template and suitable organic precursors. Pt NPs were deposited by solid-state reduction of platinum acetylacetonate under N2/H2 flow on the three different supports. Pt NPs resulted to be well-dispersed over the doped MC supports with size distributions (from 1.8 nm to 3.5 nm) that are dependent on the type of doping heteroatom (N, S, or N and S). The influence of nitrogen and/or sulfur incorporated into the carbon matrix on the nucleation and growth of Pt NPs was also rationalized based on density functional theory (DFT) simulations. They highlighted that both nitrogen and sulfur increase the interactions between Pt and carbon support, but the interaction decreases as the nitrogen an...