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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Li, Chen
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (10/10 displayed)
- 2022Shuffling Atomic Layer Deposition Gas Sequences to Modulate Bimetallic Thin Films and Nanoparticle Propertiescitations
- 2022Shuffling atomic layer deposition gas sequences to modulate bimetallic thin films and nanoparticle propertiescitations
- 2021Grain boundaries as a diffusion-limiting factor in lithium-rich NMC cathodes for high-energy lithium-ion batteriescitations
- 2020Near-Edge Ligand Stripping and Robust Radiative Exciton Recombination in CdSe/CdS Core/Crown Nanoplateletscitations
- 2020Developing Lattice Matched ZnMgSe Shells on InZnP Quantum Dots for Phosphor Applicationscitations
- 2020Developing Lattice Matched ZnMgSe Shells on InZnP Quantum Dots for Phosphor Applicationscitations
- 2020Near-edge ligand stripping and robust radiative exciton recombination in CdSe/CdS core/crown nanoplateletscitations
- 2016nitial Cumulative Effects in Femtosecond Pulsed Laser-induced Periodic Surface Structures on Bulk Metallic Glassescitations
- 2016Scattering effects and high-spatial-frequencynanostructures on ultrafast laser irradiatedsurfaces of zirconium metallic alloys with nanoscaledtopographiescitations
- 2014A study of photothermal laser ablation of various polymers on microsecond time scalescitations
Places of action
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article
Developing Lattice Matched ZnMgSe Shells on InZnP Quantum Dots for Phosphor Applications
Abstract
<p>Indium phosphide quantum dots (QDs) have drawn attention as alternatives to cadmium- and lead-based QDs that are currently used as phosphors in lamps and displays. The main drawbacks of InP QDs are, in general, a lower photoluminescence quantum yield (PLQY), a decreased color purity, and poor chemical stability. In this research, we attempted to increase the PLQY and stability of indium phosphide QDs by developing lattice matched InP/MgSe core-shell nanoheterostructures. The choice of MgSe comes from the fact that, in theory, it has a near-perfect lattice match with InP, provided MgSe is grown in the zinc blende crystal structure, which can be achieved by alloying with zinc. To retain lattice matching, we used Zn in both the core and shell and we fabricated InZnP/Zn<sub>x</sub>Mg<sub>1-x</sub>Se core/shell QDs. To identify the most suitable conditions for the shell growth, we first developed a synthesis route to Zn<sub>x</sub>Mg<sub>1-x</sub>Se nanocrystals (NCs) wherein Mg is effectively incorporated. Our optimized procedure was employed for the successful growth of Zn<sub>x</sub>Mg<sub>1-x</sub>Se shells around In(Zn)P QDs. The corresponding core/shell systems exhibit PLQYs higher than those of the starting In(Zn)P QDs and, more importantly, a higher color purity upon increasing the Mg content. The results are discussed in the context of a reduced density of interface states upon using better lattice matched Zn<sub>x</sub>Mg<sub>1-x</sub>Se shells.</p>