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Casey, Abby
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article
Vinylene-Linked Oligothiophene-Difluorobenzothiadiazole Copolymer for Transistor Applications
Abstract
<p>The synthesis of the novel donor-acceptor monomer 4,7-bis[(E)-2-(5-bromo-3-dodecylylthiophen-2-yl)ethenyl]-5,6-difluoro-2,1,3-benzothiadiazole (FBT-V2T2) is reported. Polymerization with 4,4′-ditetradecyl-5,5′-bistrimethylstannyl-2,2′-bithiophene afforded a highly crystalline polymer that aggregated strongly in solution. Polymer films were well ordered resulting in high performance field-effect transistors with low onset voltages, negligible hysteresis, high channel current on/off ratios, and peak hole mobilities of up to 0.5 cm<sup>2</sup> V<sup>-1</sup> s<sup>-1</sup>. Notably the transistors exhibited close to ideal behavior with extracted mobilities almost independent of gate of voltage.</p>