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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Valev, Vk
University of Bath
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (9/9 displayed)
- 2019WS2 Nanotubes, 2D Nanomeshes, and 2D In-Plane Films Through One Single Chemical Vapor Deposition routecitations
- 2019Second harmonic spectroscopy of surface lattice resonancescitations
- 2014Ultrafast nonlinear response of gold gyroid three-dimensional metamaterialscitations
- 2014Layer-by-Layer synthesis and tunable optical properties of hybrid magnetic-plasmonic nanocomposites using short bifunctional molecular linkerscitations
- 2013Magneto-optical harmonic susceptometry of superparamagnetic materialscitations
- 2012Characterization of magnetization-induced second harmonic generation in iron oxide polymer nanocompositescitations
- 2011Si passivation for Ge pMOSFETscitations
- 2011Adsorption kinetics of ultrathin polymer films in the melt probed by dielectric spectroscopy and second-harmonic generationcitations
- 2011Preparing polymer films doped with magnetic nanoparticles by spin-coating and melt-processing can induce an in-plane magnetic anisotropycitations
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article
Second harmonic spectroscopy of surface lattice resonances
Abstract
Because of their large figures of merit, surface lattice resonances (SLRs) in metal nanoparticle arrays are very promising for chemical and biomolecular sensing in both liquid and gas media. SLRs are sensitive to refractive index changes both near the surface of the nanoparticles (surface sensitivity) and in the volume between them (bulk sensitivity). Because of its intrinsic surface-sensitivity and a power law dependence on electric fields, second harmonic generation (SHG) spectroscopy can improve upon both the surface and volume sensitivities of SLRs. In this report on SHG spectroscopy of plasmonic nanoparticles, we show that the SHG signal is greatly increased (up to 450 times) by the SLRs. We also demonstrate very narrow resonances in SHG intensity (∼5 nm fwhm). We illustrate how the SHG resonances are highly sensitive to SLRs by varying the fundamental wavelength, angle of incidence, nanoparticle material, and lattice constant of the arrays. Finally, we identify an SHG resonance (10 nm fwhm) that is electric dipole forbidden and can be attributed to higher-order multipoles, enhanced by the strong near-fields of SLRs. Our results open up new and very promising avenues for chemical and biomolecular sensing based on SHG spectroscopy of SLRs.