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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Meunier, V.
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Topics
Publications (8/8 displayed)
- 2024Operando observation of the dynamic SEI formation on a carbonaceous electrode by near-ambient pressure XPScitations
- 2022Electron–Phonon Coupling in a Magic-Angle Twisted-Bilayer Graphene Device from Gate-Dependent Raman Spectroscopy and Atomistic Modelingcitations
- 2020Massive Dirac Fermion Behavior in a Low Bandgap Graphene Nanoribbon Near a Topological Phase Boundary.citations
- 2019An unexpected organometallic intermediate in surface-confined Ullmann couplingcitations
- 2016Quasi one-dimensional band dispersion and surface metallization in long-range ordered polymeric wirescitations
- 2013Insight into organometallic intermediate and its evolution to covalent bonding in surface-confined ullmann polymerizationcitations
- 2012Nanoscale ferroelectricity in crystalline γ-glycinecitations
- 2003Fullerenes coalescence in nanopeapods : a path to novel tubular carboncitations
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article
Electron–Phonon Coupling in a Magic-Angle Twisted-Bilayer Graphene Device from Gate-Dependent Raman Spectroscopy and Atomistic Modeling
Abstract
The importance of phonons in the strong correlation phenomena observed in twisted-bilayer graphene (TBG) at the so-called magic-angle is under debate. Here we apply gate-dependent micro-Raman spectroscopy to monitor the G band line width in TBG devices of twist angles ! = 0° (Bernal), "1.1° (magic-angle), and "7° (large-angle). The results show a broad and p-/n-asymmetric doping behavior at the magic angle, in clear contrast to the behavior observed in twist angles above and below this point. Atomistic modeling reproduces the experimental observations in close connection with the joint density of electronic states in the electron−phonon scattering process, revealing how the unique electronic structure of magic-angle TBGs influences the electron−phonon coupling and, consequently, the G band line width. Overall, the value of the G band line width in magic-angle TBG is larger when compared to that of the other samples, in qualitative agreement with our calculations.