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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Konstas, Kristina
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (9/9 displayed)
- 2022Charge carrier molecular sieve (CCMS) membranes with anti-aging effect for long-life vanadium redox flow batteriescitations
- 2020Engineered Porous Nanocomposites That Deliver Remarkably Low Carbon Capture Energy Costscitations
- 2019Thermally Rearranged Mixed Matrix Membranes (TR-MMM) for Permeability Enhancement and Mechanical Toughnesscitations
- 2017Post-Synthetic Annealing: Linker Self-Exchange in UiO-66 and its Effect on Polymer-MOF Interactioncitations
- 2017Materials Genome in Action: Identifying the Performance Limits of Physical Hydrogen Storagecitations
- 2016Physical aging in glassy mixed matrix membranes; tuning particle interaction for mechanically robust nanocomposite filmscitations
- 2015Lead(II) uptake by aluminium based magnetic framework composites (MFCs) in watercitations
- 2012Methane storage in metal organic frameworkscitations
- 2012Magnetic framework composites for polycyclic aromatic hydrocarbon sequestrationcitations
Places of action
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article
Engineered Porous Nanocomposites That Deliver Remarkably Low Carbon Capture Energy Costs
Abstract
A key barrier to the use of carbon dioxide capture technologies is the operating energy requirement, the chief contributor being the energy required to regenerate the capture media. When paired with electricity generation, the parasitic energy load can prohibit implementation. While metal organic frameworks (MOFs) harbor significant adsorption capacities, their thermally insulating nature will require significant energy and time to regenerate. Here, we report a MOF nanocomposite that can be regenerated at high speed and low energy cost. An adsorption system is tailored to deliver a very low energy cost of only 1.29 MJ kg−1CO2, 45% below commercially deployed materials, which can be exploited to deliver a productivity as high as 3.13 kgCO2 h−1 kgAds−1. The combination of a MOF (Mg-MOF-74) with high adsorption capacity, a magnetic nanoparticle (MgFe2O4), and a porous hydrophobic polymer results in a composite that can be used in the magnetic induction swing adsorption (MISA) process.