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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Ruseckas, Arvydas
University of St Andrews
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (20/20 displayed)
- 2023Chlorine retention enables the indoor light harvesting of triple halide wide bandgap perovskitescitations
- 2020Efficient indoor p-i-n hybrid perovskite solar cells using low temperature solution processed NiO as hole extraction layerscitations
- 2020Low threshold polariton lasing from a solution-processed organic semiconductor in a planar microcavitycitations
- 2019Efficient indoor p-i-n hybrid perovskite solar cells using low temperature solution processed NiO as hole extraction layerscitations
- 2019Low threshold polariton lasing from a solution-processed organic semiconductor in a planar microcavitycitations
- 2019Efficient indoor pin hybrid perovskite solar cells using low temperature solution processed NiO as hole extraction layerscitations
- 2019Improved efficiency of PbS quantum dot sensitized NiO photocathodes with naphthalene diimide electron acceptor bound to the surface of the nanocrystalscitations
- 2019Interface limited hole extraction from methylammonium lead iodide filmscitations
- 2019Interface limited hole extraction from methylammonium lead iodide filmscitations
- 2019Hole delocalization as a driving force for charge pair dissociation in organic photovoltaicscitations
- 2018Improved efficiency of PbS quantum dot sensitized NiO photocathodes with naphthalene diimide electron acceptor bound to the surface of the nanocrystalscitations
- 2017Tuning crystalline ordering by annealing and additives to study its effect on exciton diffusion in a polyalkylthiophene copolymercitations
- 2016Self-trapping and excited state absorption in fluorene homo-polymer and copolymers with benzothiadiazole and tri-phenylaminecitations
- 2015Controlling exciton diffusion and fullerene distribution in photovoltaic blends by side chain modificationcitations
- 2012Nanosecond two-photon absorption and lasing in fluorene-based organic semiconductors
- 2012A Shift from Diffusion Assisted to Energy Transfer Controlled Fluorescence Quenching in Polymer-Fullerene Photovoltaic Blendscitations
- 2009A two-photon pumped polyfluorene lasercitations
- 2009Effects of thermal annealing on the photophysical properties of bisfluorene-cored dendrimer filmscitations
- 2008Thickness Dependence of the Fluorescence Lifetime in Films of Bisfluorene-Cored Dendrimerscitations
- 2008Distance dependence of excitation energy transfer between spacer-separated conjugated polymer filmscitations
Places of action
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article
Efficient indoor pin hybrid perovskite solar cells using low temperature solution processed NiO as hole extraction layers
Abstract
Hybrid perovskites have received tremendous attention due to their exceptional photovoltaic and optoelectronic properties. Among the two widely used perovskite solar cell device architectures of n-i-p and p-i-n, the latter is interesting in terms of its simplicity of fabrication and lower energy input. However this structure mostly uses PEDOT:PSS as a hole transporting layer which can accelerate the perovskite solar cell degradation. Hence the development of stable, inorganic hole extraction layers (HEL), without compromising the simplicity of device fabrication is crucial in this fast-growing photovoltaic field. Here we demonstrate a low temperature (~100 oC) solution - processed and ultrathin (~ 6 nm) NiO nanoparticle thin film as an efficient HEL for CH3NH3PbI3 based perovskite solar cells. We measure a power conversion efficiency (PCE) of 13.3 % on rigid glass substrates and 8.5 % on flexible substrates. A comparison with PEDOT:PSS based MAPbI3solar cells (PCE ~ 7.9 %) shows that NiO based solar cells have higher short circuit current density and improved open circuit voltage (1.03V).Apart from the photovoltaic performance under 1 Sun, the efficient hole extraction property of NiO is demonstrated for indoor lighting as well with a PCE of 23.0 % for NiO based CH3NH3PbI2.9Cl0.1 p-i-n solar cells under compact fluorescent lighting. Compared to the perovskite solar cells fabricated on PEDOT:PSS HEL, better shelf-life stability is observed for perovskite solar cells fabricated on NiO HEL. Detailed microstructural and photophysical investigations imply uniform morphology, lower recombination losses, and improved charge transfer properties for CH3NH3PbI3grown on NiO HEL.