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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Cretin, Marc
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (20/20 displayed)
- 2024Cobalt-substituted porous calcium copper titanate electrodes for paracetamol degradation by an electro-oxidation/peroxymonosulfate systemcitations
- 2024Cobalt-substituted porous calcium copper titanate electrodes for paracetamol degradation by an electro-oxidation/peroxymonosulfate system
- 2023A novel BN/TiO2/HNT nanocomposite for photocatalytic applications fabricated by electrospinningcitations
- 2023N-Doped HNT/TiO2 Nanocomposite by Electrospinning for Acetaminophen Degradationcitations
- 2023N-Doped HNT/TiO2 Nanocomposite by Electrospinning for Acetaminophen Degradationcitations
- 2023A facile approach to modify cellulose nanocrystal for the adsorption of perfluorooctanoic acidcitations
- 2023A Comprehensive Review on Modification of Titanium Dioxide‐Based Catalysts in Advanced Oxidation Processes for Water Treatmentcitations
- 2023Photoelectrocatalytic Degradation of Methylene Blue on Electrodeposited Bismuth Ferrite Perovskite Filmscitations
- 2022Recent progress on chemical modification of cellulose nanocrystal (CNC) and its application in nanocomposite films and membranes-A comprehensive reviewcitations
- 2022Detailed manufacturing process of a tubular carbon microfiltration membrane for industrial wastewater treatmentcitations
- 2022Electrochemical oxidation treatment of Direct Red 23 aqueous solutions: Influence of the operating conditionscitations
- 2021Synthesis and Characterization of Activated Carbon Co-Mixed Electrospun Titanium Oxide Nanofibers as Flow Electrode in Capacitive Deionizationcitations
- 2021Photoelectrocatalysis of paracetamol on Pd–ZnO/ N-doped carbon nanofibers electrodecitations
- 2020Highly efficient and stable FeIIFeIII LDH carbon felt cathode for removal of pharmaceutical ofloxacin at neutral pHcitations
- 2020Coupling cathodic electro-fenton with anodic photo-electrochemical oxidation: A feasibility study on the mineralization of paracetamolcitations
- 2019Hybrid graphene-decorated metal hollow fibre membrane reactors for efficient electro-Fenton - Filtration co-processescitations
- 2019Hybrid graphene-decorated metal hollow fibre membrane reactors for efficient electro-Fenton - Filtration co-processescitations
- 2017Surfactant- and Binder-Free Hierarchical Platinum Nanoarrays Directly Grown onto a Carbon Felt Electrode for Efficient Electrocatalysiscitations
- 2016Facile Preparation of Porous Carbon Cathode to Eliminate Paracetamol in Aqueous Medium Using Electro-Fenton Systemcitations
- 2008Surface Modifications of Love Acoustic Waves Sensors for Chemical and Biological Detection
Places of action
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article
Hybrid graphene-decorated metal hollow fibre membrane reactors for efficient electro-Fenton - Filtration co-processes
Abstract
Metal hollow fibre membranes offer excellent chemical and mechanical stability and are promising platforms for the removal of harsh contaminants from solutions. Stainless steel (SS) membranes are however prone to oxidation and advanced decoration routes are required to passivate the surface of such materials. Here, SS membranes were modified with nanoscale coatings of graphene to promote electrochemical reactions and prevent premature corrosion of the bare metal reinforcement upon electro-Fenton (EF) reaction. Samples decorated with graphene oxide or reduced graphene oxide were compared to bare SS membranes to assess the impact of graphitization on the electrochemical performance of the membranes. Membranes properties were characterized using both cyclic and linear scanning voltammetry. The results evidenced that electron transfer kinetics were significantly enhanced on the reduced graphene oxide, compared to raw material. In addition, the removal efficiency of a pharmaceutical pollutant, paracetamol, was evaluated in electro-Fenton batch experiments, on the three membrane electrodes. The best mineralization current efficiency at 37% was found when using reduced graphene oxide membrane cathode at optimal applied potential of -0.5 V vs. SCE (Saturated Calomel Electrode). Finally, the coupling of electro-Fenton and filtration processes was carried out on a pilot-scale unit. Various electrochemical and hydrodynamic parameters that affect mineralization efficiency were studied. By coupling filtration and electrochemical processes, the mineralization current efficiency value was increased remarkably by 165% and remained stable for three consecutive cycles. This strategy opens up opportunities to generate low cost catalytic membrane reactors with high flux and selectivity from the materials reactivity as opposed to sieving, with potential for harsh chemicals mineralization.