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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Osenberg, Markus
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (14/14 displayed)
- 2024Opportunities and Challenges of Calendering Sulfide‐Based Separators for Solid‐State Batteriescitations
- 2023Roadmap for focused ion beam technologiescitations
- 2023Roadmap for focused ion beam technologiescitations
- 2023Unveiling the impact of cross-linking redox-active polymers on their electrochemical behavior by 3D imaging and statistical microstructure analysiscitations
- 20223D microstructure characterization of polymer battery electrodes by statistical image analysis based on synchrotron X-ray tomographycitations
- 2022Fabrication and characterization of porous mullite ceramics derived from fluoride-assisted Metakaolin-Al(OH)3 annealing for filtration applications
- 2021Stochastic 3D microstructure modeling of anodes in lithium-ion batteries with a particular focus on local heterogeneitycitations
- 2021Hierarchical Structuring of NMC111-Cathode Materials in Lithium-Ion Batteries: An In-Depth Study on the Influence of Primary and Secondary Particle Sizes on Electrochemical Performance
- 2020Hierarchical Structuring of NMC111-Cathode Materials in Lithium-Ion Batteries: An In-Depth Study on the Influence of Primary and Secondary Particle Sizes on Electrochemical Performancecitations
- 2020X‐Ray‐Computed Radiography and Tomography Study of Electrolyte Invasion and Distribution inside Pristine and Heat‐Treated Carbon Felts for Redox Flow Batteries
- 2020Hierarchical Structuring of NMC111-Cathode Materials in Lithium-Ion Batteriescitations
- 2019On a pluri-Gaussian model for three-phase microstructures, with applications to 3D image data of gas-diffusion electrodescitations
- 2019X‐ray‐computed radiography and tomography study of electrolyte invasion and distribution inside pristine and heat‐treated carbon felts for redox flow batteries
- 2018Correlating Morphological Evolution of Li Electrodes with Degrading Electrochemical Performance of Li/LiCoO2 and Li/S Battery Systemscitations
Places of action
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article
3D microstructure characterization of polymer battery electrodes by statistical image analysis based on synchrotron X-ray tomography
Abstract
Polymer-based batteries represent a promising concept for next-generation energy storage due to their potentially higher power densities and smaller ecological footprint, compared to classical Li-ion batteries. Since the microstructure of electrodes is a key factor for the performance of battery cells, a detailed understanding of this microstructure is essential for the improvement of manufacturing processes. In the present contribution, the 3D microstructure of electrodes for polymer-based batteries is quantitatively characterized for the first time, where synchrotron X-ray tomography is combined with statistical image analysis. In particular, 3D imaging is performed for two porous electrodes, which both consist of the redox-active polymer PTMA as well as conductive additives, but differ regarding their binder materials. The focus is put on local heterogeneity of volume fractions of the constituents, surface area per unit volume of the polymer phase and the length of shortest transportation paths through both, polymer and binder-additive phase. It is shown that using different binder materials leads to significant differences regarding the 3D electrode microstructures. In this way, statistical analysis of image data helps to gain further insight into the influence of manufacturing processes on electrode microstructures and thus, on the performance of battery cells.