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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Kazansky, Peter
University of Southampton
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (41/41 displayed)
- 2017Ultrafast laser-induced birefringence in various porosity silica glasses: from fused silica to aerogelcitations
- 2015Functional birefringent elements imprinted by femtosecond laser nanostructuring of multi-component glass
- 2015Revealing the nanoparticles aspect ratio in the glass-metal nanocomposites irradiated with femtosecond lasercitations
- 2015Glass-metal nanocomposite modification by femtosecond laser irradiation
- 2014High-purity, broadband, entangled photon pairs generated in poled silica fibers
- 2014Multi-watt all-fiber frequency doubled lasercitations
- 2014All-fiber frequency-doubled visible lasercitations
- 2013Extraordinary anisotropy of ultrafast laser writing in glasscitations
- 2013Laser assisted modification of poled silver-doped nanocomposite soda-lime glass
- 2012Exciton mediated self-organization in glass driven by ultrashort light pulsescitations
- 2011Light coupling and enhanced backscattering in layered plasmonic nanocompositescitations
- 2011Type II parametric downconversion in a poled fiber
- 2010Measurement of X(2) symmetry in a poled fibercitations
- 2010Enhanced light backscattering in thermally poled plasmonic nanocomposite and its application to vapour sensing
- 2010Leaky-modes excitation in thermally poled nanocomposite glass and their exploitation for saturable absorption
- 2010Saturation of absorption in noble metal doped nanocomposite glass film excited by evanescent light fieldcitations
- 2010Poling-assisted fabrication of plasmonic nanocomposite devices in glasscitations
- 2010The problem of achieving high second-order nonlinearities in glasses: The role of electric conductivity in poling of high index glassescitations
- 2010Aperiodically poled silica fibers for bandwidth control of quasi-phase-matched second-harmonic generationcitations
- 2009From type II upconversion to SPDC: a path to broadband polarization entanglement in poled fibers
- 2009High-average-power second-harmonic generation from periodically poled silica fiberscitations
- 2008Low loss photonic components in high index bismuth borate glass by femtosecond laser direct writingcitations
- 2008Ion-exchange-induced formation of glassy electrooptical and nonlinear optical nanomaterialcitations
- 2007Broadly tunable second-harmonic generation in periodically poled silica fiberscitations
- 2007Photon pair source based on parametric fluorescence in periodically poled twin-hole silica fibercitations
- 2007Recent advances in poling and nanostructuring of glass
- 2007Dissolution of embedded gold nanoparticles in sol-gel glass filmcitations
- 2006Creating unusual structures by ultrashort light pulses in glass
- 2006Bleaching of sol-gel glass film with embedded gold nanoparticles by thermal polingcitations
- 2006Breaking symmetry in glass by femtosecond laser irradiation
- 2005Electric field-assisted formation of percolated silver nanolayers inside glasscitations
- 2005Refractive index engineering in glass containing spherical silver nanoparticles using dc electric field
- 2005Origin and enhancement of the second-order non-linear optical susceptibility induced in bismuth borate glasses by thermal polingcitations
- 2004Enhanced stability of the second-order optical nonlinearity in poled glassescitations
- 2004Optical waveguides in electrooptical nanophase glass-ceramicscitations
- 2002Nonlinearity in poled tin-doped silica samples fabricated by sol-gel technique
- 2002Femtosecond laser direct-writing and poling of embedded grating structures
- 2001UV laser-induced current in germanosilicate fibres with built in electrodes
- 2001Thermally poled silica samples are structurally heterogeneous: Electron diffraction evidence of partial crystallizationcitations
- 2000Propagation of cold atoms along a miniature magnetic guidecitations
- 2000Memorized polarization-dependent light scattering in rare-earth-ion-doped glasscitations
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article
Origin and enhancement of the second-order non-linear optical susceptibility induced in bismuth borate glasses by thermal poling
Abstract
The second-order non-linear optical susceptibility of thermally poled glasses, chi(2), should be enhanced in proportion to the intrinsic third-order susceptibility chi(3), for a given frozen-in electric field (i.e. chi(2) = 3Edcchi(3)). In order to test this prediction, bismuth-borate (Bi2O3–ZnO–B2O3) glasses, for which chi(3) increased with increasing Bi2O3 content, were thermally poled and the second-order non-linear coefficient was determined. Poling conditions and current dynamics turned out to be very different from those in silica. Poling temperatures had to be relatively close to glass transition temperatures and the glass–electrode contact had to be intimate in order to induce the non-linearity which was located in a near-surface layer at the anode side. A poling mechanism was proposed which relied on proton migration, took into account ion injection and glass ionization, and was able to explain most of the experimental results. The chi(2) values increased with increasing chi(3) as predicted but did not exceed 0.7 pm/V. By comparison with silica, it was inferred that the dielectric breakdown strength Eb was lower in bismuth borate and decreased with increasing Bi2O3 content. This latter result demonstrated the importance to select glass compositions on the basis of both chi(3) and Eb for the purpose of enhancing chi(2).