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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Asgari, Asgari
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (12/12 displayed)
- 2024The first proof-of-concept of straightforward and ambient-processed CsPbBr3 perovskite light-emitting electrochemical cellcitations
- 2024High-performance semi-transparent organic solar cells for window applications using MoO3/Ag/MoO3 transparent anodescitations
- 2024Enhancing Efficiency of Luminescent Solar Concentrators through Laser Grooving Techniques
- 2024Enhanced performance of ambient-air processed CsPbBr3 perovskite light-emitting electrochemical cells via synergistic incorporation of dual additivescitations
- 2023Nitride/Perovskite Tandem Solar Cell with High Stabilitycitations
- 2023Improving phototransistor performance with polymer-quantum dot hybrid technologycitations
- 2023The role of domain size and weight ratio of fullerene and non-fullerene acceptors on performance of PM6:Y6citations
- 2021Perovskite-coated window glasses as semi-transparent luminescent solar concentratorscitations
- 2021Fabrication of a light-emitting device based on the CdS/ZnS spherical quantum dotscitations
- 2020The improved performance of BHJ organic solar cells by random dispersed metal nanoparticles through the active layercitations
- 2018Radiation characteristics of Leaky Surface Plasmon polaritons of graphenecitations
- 2017Modeling and optimizing the performance of plasmonic solar cells using effective medium theorycitations
Places of action
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article
Enhanced performance of ambient-air processed CsPbBr3 perovskite light-emitting electrochemical cells via synergistic incorporation of dual additives
Abstract
<p>Metal halide perovskite light-emitting electrochemical cells (MHP-LECs) are promising due to their facile solution processability and exceptional optoelectrical properties. However, commercialization is hindered by poor thin-film coverage and the need for glovebox processing. This study addresses these issues by incorporating poly(ethylene oxide) (PEO) and potassium hexafluorophosphate (KPF<sub>6</sub>) into cesium lead bromide perovskite (CsPbBr<sub>3</sub>) emitting layers (EML), processed under ambient-air conditions. These perovskite composite thin films were spin-coated on a preheated substrate, and the device structure was ITO/PEDOT:PSS/EML/Al. Notably, the MHP-LEC based on CsPbBr<sub>3</sub>:PEO:KPF<sub>6</sub> (100:65:0.2, weight ratio) exhibited pure-green emission with a peak at 524 nm and a narrow full width at half-maximum of 27 nm. Compared to a reference device (CsPbBr<sub>3</sub>:PEO (100:65, weight ratio)), the new device showed 1.5-, 4-, and 5-fold improvements in current density, electroluminescence (EL) intensity, and lifetime, respectively. These enhancements are attributed to reduced non-radiative current leakage, improved film surface coverage and passivation, and balanced charge carrier injection and transportation. This study offers a straightforward approach for processing CsPbBr<sub>3</sub> thin films under ambient-air conditions, enhancing the EL performance of MHP-LECs.</p>