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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Jagadamma, Lethy Krishnan
University of St Andrews
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (21/21 displayed)
- 2024Metal oxide vs organic semiconductor charge extraction layers for halide perovskite indoor photovoltaics
- 2023Manipulation of structure and optoelectronic properties through bromine inclusion in a layered lead bromide perovskitecitations
- 2023Chlorine retention enables the indoor light harvesting of triple halide wide bandgap perovskitescitations
- 2023Lead-free perovskite-inspired semiconductors for indoor light-harvesting - the present and the futurecitations
- 2023Status report on emerging photovoltaicscitations
- 2022Crystalline grain engineered CsPbIBr2 films for indoor photovoltaicscitations
- 2022Solution-processable perylene diimide-based electron transport materials as non-fullerene alternatives for inverted perovskite solar cellscitations
- 2022Solution-processable perylene diimide-based electron transport materials as non-fullerene alternatives for inverted perovskite solar cellscitations
- 2022Hysteresis in hybrid perovskite indoor photovoltaicscitations
- 2021Organic photovoltaics for simultaneous energy harvesting and high-speed MIMO optical wireless communicationscitations
- 2021New thiophene-based conjugated macrocycles for optoelectronic applicationscitations
- 2021New thiophene-based conjugated macrocycles for optoelectronic applicationscitations
- 2019Efficient indoor pin hybrid perovskite solar cells using low temperature solution processed NiO as hole extraction layerscitations
- 2019Interface limited hole extraction from methylammonium lead iodide filmscitations
- 2017Charge carrier localised in zero-dimensional (CH3NH3)3Bi219 clusterscitations
- 2017Charge carrier localised in zero-dimensional (CH3NH3)3Bi2I9 clusterscitations
- 2017Novel 4,8-benzobisthiazole copolymers and their field-effect transistor and photovoltaic applicationscitations
- 2016Solution-processable MoO x nanocrystals enable highly efficient reflective and semitransparent polymer solar cellscitations
- 2016Solution-processable MoOx nanocrystals enable highly efficient reflective and semitransparent polymer solar cellscitations
- 2015Polymer solar cells with efficiency >10% enabled via a facile solution-processed Al-doped ZnO electron transporting layercitations
- 2015Polymer solar cells with efficiency >10% enabled via a facile solution-processed Al-doped ZnO electron transporting layercitations
Places of action
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article
Crystalline grain engineered CsPbIBr2 films for indoor photovoltaics
Abstract
Indoor photovoltaic devices have garnered profound research attention in recent years due to their prospects of powering ‘smart’ electronics for the Internet of Things (IoT). Here it is shown that all-inorganic Cs-based halide perovskites are promising for indoor light harvesting due to their wide bandgap matched to the indoor light spectra. Highly crystalline and compact CsPbIBr<sub>2</sub> perovskite based photovoltaic devices have demonstrated a power conversion efficiency (PCE) of 14.1% under indoor illumination of 1000 lx and 5.9% under 1 Sun. This study revealed that a reduction in grain misorientation, as well as suppression of defects in the form of metallic Pb in the perovskite film are crucial for maximising the photovoltaic properties of CsPbIBr<sub>2</sub> based devices. It was demonstrated that a pinhole free CsPbIBr<sub>2</sub>/Spiro-OMeTAD interface preserves the perovskite α phase and enhances the air stability of the CsPbIBr<sub>2</sub> devices. These devices, despite being unencapsulated, retained > 55% of the maximum PCE even when stored under 30% relative humidity for a shelf-life duration of 40 days and is one of the best stability data reported so far for CsPbIBr<sub>2</sub> devices.