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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Achour, Amine
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (8/8 displayed)
- 2023Plasma Treatment of Polystyrene Films—Effect on Wettability and Surface Interactions with Au Nanoparticlescitations
- 2022Low-pressure plasma process for the dry synthesis of cactus-like Au-TiO2 nanocatalysts for toluene degradationcitations
- 2022X-ray Photoelectron Spectroscopy (XPS) Analysis of Ultrafine Au Nanoparticles Supported over Reactively Sputtered TiO 2 Filmscitations
- 2022Low-pressure plasma process for the dry synthesis of cactus-like Au-TiO 2 nanocatalysts for toluene degradationcitations
- 2019Correlation between surface topography, optical band gaps and crystalline properties of engineered AZO and CAZO thin filmscitations
- 2015AlN films deposited by dc magnetron sputtering and high power impulse magnetron sputtering for SAW applicationscitations
- 2014Achieving high thermal conductivity from AlN films deposited by high-power impulse magnetron sputteringcitations
- 2014Achieving high thermal conductivity from AlN films deposited by high-power impulse magnetron sputteringcitations
Places of action
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article
Low-pressure plasma process for the dry synthesis of cactus-like Au-TiO2 nanocatalysts for toluene degradation
Abstract
<p>The development of environment-friendly, low-cost and efficient catalyst preparation processes has always been a major issue in the field of catalysis. Wet chemistry methods are often used but these techniques are not sustainable, as post waste solution treatment remains an important drawback. Here an innovative dry low-pressure plasma process for metal nanoparticles supported nanocatalysts preparation is reported. The solid metal and oxide support precursors are physically mixed and then exposed to a radiofrequency Ar/N<sub>2</sub> plasma discharge, leading to the precursor degradation and the subsequent nanoparticles generation, without pre- or post- preparation steps. The metal nanoparticle loading and the particle size of metal and oxide support can be easily tuned by changing the ratio of the precursor materials, making the process simple, versatile, highly efficient, and scalable. As a proof of concept, gold nanoparticles (Au NPs) supported on titanium dioxide (TiO<sub>2</sub>) were prepared and tested as nanocatalysts for toluene (C<sub>7</sub>H<sub>8</sub>) degradation at temperatures ranging from 25 to 450 °C. Up to 100% of C<sub>7</sub>H<sub>8</sub> conversion into CO<sub>2</sub> was achieved over the Au-TiO<sub>2</sub> nanocatalysts, demonstrating that this dry method is a very efficient way to prepare highly active nanocatalysts.</p>